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Optica Publishing Group
  • Chinese Optics Letters
  • Vol. 8,
  • Issue 7,
  • pp. 683-684
  • (2010)

Photoluminescence study of the annihilation process of donor-bound excitons in ZnO: observation of quantum mechanical interference

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Abstract

We report a photoluminescence observation of the coupling of donor-bound excitons and longitudinal optical phonons in high-quality ZnO crystals at 5 K. The first-order phonon Stockes line of donor-bound excitons exhibits a distinct asymmetric line shape with a clear dip at its higher energy side, suggesting that quantum mechanical interference occurs during the annihilation of donor-bound excitons. The donor binding energy is determined to be 49.3 meV from spectral featural.

© 2010 Chinese Optics Letters

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