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Multidimensional Stimulated Resonant Raman X-ray Spectroscopy of Molecules

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Abstract

Valence excitations can be studied by watching wavepackets launched by sequences of attosecond x-ray pulses. This is is demonstrated by simulations for trans-N-methylacetamide (NMA) at the oxygen and nitrogen K-edges. A Super Magic Angle (SMA) combination of two measurements with specific pulse polarization configurations can simplify the interpretation of these signals.

© 2012 Optical Society of America

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