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Single Molecule Pump-Probe Detection on Coupled Quantum Systems

N.F. van Hulst, E.M.H.P. van Dijk, J.P. Hoogenboom, J. Hernando, and M.F. Garcia-Parajo

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Abstract

We present a single-molecule study on exciton dynamics in multichromophoric systems, combining fs pump-probe, emission-spectra and fluorescence-lifetime analysis. A wide range of static disorder and exciton delocalisation accelerates dephasing and relaxation rate of the exciton.

© 2006 Optical Society of America

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