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2D-IR Photon Echo Spectroscopy of Pure Liquid Water - Combination of Novel Nanofluidics and Diffractive Optics Deciphers Ultrafast Structural Dynamics

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Abstract

2D-IR photon echo studies of the OH stretching vibration in pure liquid water are presented. At room temperature, a 50-fs decay of structural correlations is found. The temperature dependence of the vibrational dynamics is investigated.

© 2006 Optical Society of America

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