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Mechanism of radical transfer during photoactivation of the flavoprotein DNA photolyase

Andras Lukacs, Marten H. Vos, André P. M. Eker, Martin Byrdin, and Klaus Brettel

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Abstract

Ultrafast transient absorption experiments on mutant DNA photolyase imply that radical transfer along a chain of tryptophan residues is substantially faster than the ~30-ps photo-induced electron-transfer event initiated by excitation of the radical flavin FADH●.

© 2006 Optical Society of America

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