Abstract

The combination of broadband pulses from a photonic crystal fiber (PCF) pumped by a standard 100 fs oscillator and pulse shaping is successfully employed for coherently controlled nonlinear spectroscopy. The pulse shaper manages not only to compress the PCF supercontinuum in a closed-loop optimization scheme but also to manipulate the phase at the same time for quantum control applications. This approach is demonstrated by single-beam coherent anti-Stokes Raman microspectroscopy and should be, due to its simplicity, well suited for general applications in nonlinear microscopy.

© 2006 Optical Society of America

Characterization of a supercontinuum generated from a photonic crystal fiber and its application to coherent Raman spectroscopy

Hideaki Kano and Hiro-o Hamaguchi
Opt. Lett. 28(23) 2360-2362 (2003)

In situ broadband pulse compression for multiphoton microscopy using a shaper-assisted collinear SPIDER

Bernhard von Vacano, Tiago Buckup, and Marcus Motzkus
Opt. Lett. 31(8) 1154-1156 (2006)

Tunable light source for coherent anti-Stokes Raman scattering microspectroscopy based on the soliton self-frequency shift

Esben Ravn Andresen, Victoria Birkedal, Jan Thøgersen, and Søren Rud Keiding
Opt. Lett. 31(9) 1328-1330 (2006)

Multiphoton intrapulse interference. IV. Ultrashort laser pulse spectral phase characterization and compensation

Vadim V. Lozovoy, Igor Pastirk, and Marcos Dantus
Opt. Lett. 29(7) 775-777 (2004)

Implementation of temporal ptychography algorithm, i²PIE, for improved single-beam coherent anti-Stokes Raman scattering measurements

Ruan Viljoen, Pieter Neethling, Dirk Spangenberg, Alexander Heidt, Hans-Martin Frey, Thomas Feurer, and Erich Rohwer
J. Opt. Soc. Am. B 37(11) A259-A265 (2020)