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Modulated conjugation as a means for attaining a record high intrinsic hyperpolarizability

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Abstract

We report on a series of chromophores that have been synthesized with a modulated conjugation path between donor and acceptor. Hyper-Rayleigh scattering measurements of the best molecule show an enhanced intrinsic hyperpolarizability that breaches the apparent limit of all previously studied molecules.

© 2006 Optical Society of America

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