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Optica Publishing Group
  • Conference on Lasers and Electro-Optics/Quantum Electronics and Laser Science and Photonic Applications Systems Technologies
  • Technical Digest (CD) (Optica Publishing Group, 2005),
  • paper JThE110

Femtosecond Hydrogen Bond Dynamics by Spectrally- and Time-Resolved Vibrational Sum Frequency Generation

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Abstract

Time- and frequency-domain 3-wave mixing spectroscopy is developed as a surface-selective nonlinear technique capable of measuring spectral evolution of vibrational coherences. Hydrogen bond dynamics of interfacial water is observed to proceed on 100 fs timescale.

© 2005 Optical Society of America

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