We demonstrate a novel technique for three-color time-resolved coherent anti-Stokes Raman scattering using a Ti:Sapphire oscillator and four-wave mixing in a photonic crystal fiber. We measure vibrational coherence decays in calcite and several molecules.
© 2007 OSA
(190.0190) Nonlinear optics : Nonlinear optics
(190.4370) Nonlinear optics : Nonlinear optics, fibers
(300.0300) Spectroscopy : Spectroscopy
(300.6230) Spectroscopy : Spectroscopy, coherent anti-Stokes Raman scattering
A. Dogariu, Y. Huang, and M. O. Scully, "Photonic Crystal Fiber Based Time-Resolved Coherent Anti-Stokes Raman Scattering Spectroscopy," in Conference on Lasers and Electro-Optics/Quantum Electronics and Laser Science Conference and Photonic Applications Systems Technologies, OSA Technical Digest Series (CD) (Optical Society of America, 2007), paper CTuA3.
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