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Reversible switching of the second-order nonlinear response

Inge Asselberghs, Koen Clays, and André Persoons

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Abstract

Reversible switching of the second-order polarisability is achieved by proton-and electron-transfer. The hyper-Rayleigh scattering technique is used to view the electronic alterations in the molecule. An azafulleroid is used for demonstrating the switching by proton-transfer, metalorganic compounds are used to show the electron-transfer switching.

© 2003 Optical Society of America

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