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Recent Advances in Two Dimensional Femtosecond Stimulated Raman Spectroscopy (2D-FSRS)

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Abstract

2D-FSRS can be implemented as either a 5th- or 7th-order nonlinear spectroscopy to probe vibrational anharmonicity with femtosecond laser pulses. Herein, we explore the effects of phasematching, concentration and pulse chirp on the Raman signal.

© 2012 Optical Society of America

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