2D-FSRS can be implemented as either a 5th- or 7th-order nonlinear spectroscopy to probe vibrational anharmonicity with femtosecond laser pulses. Herein, we explore the effects of phasematching, concentration and pulse chirp on the Raman signal.
© 2012 OSA
B. Dunlap, K. Wilson, and D. McCamant, "Recent Advances in Two Dimensional Femtosecond Stimulated Raman Spectroscopy (2D-FSRS)," in Frontiers in Optics 2012/Laser Science XXVIII, OSA Technical Digest (online) (Optical Society of America, 2012), paper LM3I.3.
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