We report the measurement of high harmonics from oriented molecules in the gas phase. We show that attosecond and re-collision science provides a detailed and sensitive probe of electronic asymmetry in polar molecules.
© 2012 OSA
(120.5050) Instrumentation, measurement, and metrology : Phase measurement
(260.1960) Physical optics : Diffraction theory
(020.2649) Atomic and molecular physics : Strong field laser physics
E. Frumker, N. Kajumba, J. Bertrand, H. Worner, C. Hebeisen, P. Hockett, M. Spanner, S. Patchkovskii, G. Paulus, D. M. Villeneuve, and P. B. Corkum, "Attosecond pulse trains generated with Oriented Molecules," in Conference on Lasers and Electro-Optics 2012, OSA Technical Digest (Optical Society of America, 2012), paper QTu1C.4.
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