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  • 14th International Conference on Ultrafast Phenomena
  • Technical Digest (CD) (Optica Publishing Group, 2004),
  • paper WA3

Measurement of Conical Intersection Dynamics by Impulsive Femtosecond Polarization Spectroscopy

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Abstract

The ~100 fs anisotropy decay from 0.4 toward 0.1 after excitation of a degenerate transition in a square molecule can be predicted from quantum beats of asymmetric vibrations and curve crossing at a conical intersection.

© 2004 Optical Society of America

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