2D-IR photon echo studies of the OH stretching vibration in pure liquid water are presented. At room temperature, a 50-fs decay of structural correlations is found. The temperature dependence of the vibrational dynamics is investigated.
© 2006 Optical Society of America
A. Paarmann, D. Kraemer, M. L. Cowan, B. D. Bruner, R. J. Miller, N. Huse, J. R. Dwyer, E. T. Nibbering, and T. Elsaesser, " 2D-IR Photon Echo Spectroscopy of Pure Liquid Water--Combination of Novel Nanofluidics and Diffractive Optics Deciphers Ultrafast Structural Dynamics," in 15th International Conference on Ultrafast Phenomena, OSA Technical Digest Series (CD) (Optical Society of America, 2006), paper MC2.
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