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Nonlinear Optical Approach to Multiexciton Relaxation Dynamics in Quantum Dots

Vanessa M. Huxter, Mayrose R. Salvador, and Gregory D. Scholes

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Abstract

We use an nth-order nonlinear transient spectroscopy to directly observe multiparticle dynamics on an ultrafast timescale in semiconductor nanocrystals. Time constants associated with multiexciton recombination and depopulation dynamics are reported.

© 2006 Optical Society of America

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