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Chirped molecular vibration after impulsive Raman excitation in a stilbene derivative molecule in solution

T. Kobayashi, A. Colonna, A. Yabushita, I. Iwakura, and E. Tokunaga

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Abstract

The vibrational dynamics in 4-methoxy-4'-nitrostilbene in a condensed phase was studied by femtosecond pump-probe spectroscopy and quantum-chemical calculation. Transient changes in absorbance due to bleaching exhibit oscillations reflecting chirped molecular vibrational on the potential surface.

© 2006 Optical Society of America

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