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Two-Photon Electronic Pump Vibrational Probe of β-apo-8’-carotenal in solution

A.J. Van Tassle, M.A. Prantil, and G.R. Fleming

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Abstract

Results of infrared transient absorption measurements following two-photon excitation to the forbidden S1 state of the carotenoid β-apo-8’-carotenal are presented. This technique enables the study of subsequent structural dynamics without interference from higher states.

© 2006 Optical Society of America

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