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Basis for ultrafast imaging of molecular orbitals with high-order harmonic generation

Tsuneto Kanai, Shinichirou Minemoto, and Hirofumi Sakai

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Abstract

We investigate ellipticity dependence of high-order harmonic generation in aligned molecules both experimentally and theoretically. Our model reproduces experimental results including geometrical and quantum interference effect and provides a basis for imaging of molecular orbitals.

© 2006 Optical Society of America

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