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Enhancement of Raman Modes in Complex Molecules by Coherent Control

J. Hauer, T. Buckup, M. Motzkus, H. Skenderovic, and K. L. Kompa

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Abstract

Using coherent control the vibrational modes in complex solvated molecules are enhanced by femtosecond pulse shaping compared to Fourier-limited excitation. The crucial role of electronic resonant transitions for the enhancement of selective states is explored.

© 2006 Optical Society of America

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