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Two Dimensional Optical Spectroscopy of Multi-Chromophore Protein Complexes

G. R. Fleming, D. Zigmantas, E. L. Read, T. Mančal, T. Brixner, and A. T. Gardiner

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Abstract

Two-dimensional optical spectroscopy is used to probe electronic couplings and ultrafast dynamics in photo synthetic light-harvesting complexes. Data and analysis reveal contributions to linebroadening, signatures of weakly- and strongly-coupled chromophores, and pathways of energy transfer.

© 2006 Optical Society of America

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