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Direct Observation of the Conical Intersection in cis-trans Photoisomerization of Rhodopsin

D. Polli, P. Altoè, O. Weingart, P. Kukura, K. M. Spillane, C. Manzoni, D. Brida, G. Tomasello, G. Orlandi, R. A. Mathies, M. Garavelli, and G. Cerullo

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Abstract

High-time-resolution broadband pump-probe spectroscopy of rhodopsin reveals loss of reactant and appearance of photoproduct features within ≈100fs, which are signatures of a wavepacket moving through a conical intersection. Experiments are supported by molecular dynamics simulations.

© 2010 Optical Society of America

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