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Applied Optics

Applied Optics

APPLICATIONS-CENTERED RESEARCH IN OPTICS

  • Vol. 36, Iss. 21 — Jul. 20, 1997
  • pp: 5168–5184

Polarized light scattering by aerosols in the marine atmospheric boundary layer

Mary S. Quinby-Hunt, Lael L. Erskine, and Arlon J. Hunt  »View Author Affiliations


Applied Optics, Vol. 36, Issue 21, pp. 5168-5184 (1997)
http://dx.doi.org/10.1364/AO.36.005168


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Abstract

The intensity and polarization of light scattered from marine aerosols affect visibility and contrast in the marine atmospheric boundary layer (MABL). The polarization properties of scattered light in the MABL vary with size, refractive index, number distributions, and environmental conditions. Laboratory measurements were used to determine the characteristics and variability of the polarization of light scattered by aerosols similar to those in the MABL. Scattering from laboratory-generated sea-salt-containing (SSC) [NaCl, (NH4)2SO4, and seawater] components of marine aerosols was measured with a scanning polarization-modulated nephelometer. Mie theory with Gaussian and log normal size distributions of spheres was used to calculate the polarized light scattering from various aerosol composition models and from experimentally determined distributions of aerosols in the marine boundary layer. The modeling was verified by comparison with scattering from distilled water aerosols. The study suggests that polarimetric techniques can be used to enhance techniques for improving visibility and remote imaging for various aerosol types, Sun angles, and viewing conditions.

© 1997 Optical Society of America

History
Original Manuscript: September 9, 1996
Revised Manuscript: February 10, 1997
Published: July 20, 1997

Citation
Mary S. Quinby-Hunt, Lael L. Erskine, and Arlon J. Hunt, "Polarized light scattering by aerosols in the marine atmospheric boundary layer," Appl. Opt. 36, 5168-5184 (1997)
http://www.opticsinfobase.org/ao/abstract.cfm?URI=ao-36-21-5168


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References

  1. G. N. Plass, T. J. Humphreys, G. W. Kattawar, “Ocean-atmosphere interface: its influence on radiation,” Appl. Opt. 20, 917–930 (1981). [CrossRef] [PubMed]
  2. G. W. Kattawar, C. N. Adams, “Stokes vector calculations of the submarine light field in an atmosphere-ocean with scattering according to a Rayleigh phase matrix: effect of interface refractive index on radiance and polarization,” Limnol. Oceanogr. 34, 1453–1472 (1989). [CrossRef]
  3. H. B. Hallock, J. Hallajian, “Polarization imaging and mapping,” Appl. Opt. 22, 964–966 (1983). [CrossRef] [PubMed]
  4. R. O. Briggs, G. L. Hatchett, “Techniques for improving underwater visibility with video equipment,” Ocean Sci. Ocean Eng. 1&2, 1284–1308 (1965).
  5. J. Cariou, B. Le Jeune, J. Lotrian, Y. Guern, “Polarization effects of seawater and underwater targets,” Appl. Opt. 29, 1689–1695 (1990). [CrossRef] [PubMed]
  6. J. E. Solomon, “Polarization mapping,” Appl. Opt. 20, 1537–1544 (1981). [CrossRef] [PubMed]
  7. G. D. Gilbert, J. C. Pernicka, “Improvement of underwater visibility by reduction of backscatter with a circular polarization technique,” in Underwater Photo-Optics Seminar Proceedings (SPIE, Santa Barbara, Calif., 1966). [CrossRef]
  8. L. E. Mertens, In-Water Photography (Wiley-Interscience, New York, 1970).
  9. P. Koepke, M. Hess, “Scattering functions of tropospheric aerosols: the effects of nonspherical particles,” Appl. Opt. 27, 2422–2430 (1988). [CrossRef] [PubMed]
  10. W. A. Hoppel, J. W. Fitzgerald, G. M. Frick, R. E. Larson, E. J. Mack, “Aerosol size distributions and optical properties found in the marine boundary layer over the Atlantic Ocean,” J. Geophys. Res. Atmos. 95D, 3659–3686 (1990). [CrossRef]
  11. J. W. Fitzgerald, “Marine aerosols—A review,” Atmos. Environ. Part A 25, 533–545 (1991). [CrossRef]
  12. D. Diermendjian, Electromagnetic Scattering on Spherical Polydispersions (American Elsevier, New York, 1969).
  13. M. S. Quinby-Hunt, P. G. Hull, A. J. Hunt, “Predicting polarization properties of marine aerosols,” in Ocean Optics XII, J. S. Jaffe, ed., Proc. SPIE2258, 735–746 (1994). [CrossRef]
  14. R. J. Perry, A. J. Hunt, D. R. Huffman, “Experimental determinations of Mueller scattering matrices for nonspherical particles,” Appl. Opt. 17, 2700–2710 (1978). [CrossRef] [PubMed]
  15. M. Z. Hansen, W. H. Evans, “Polar nephelometer for atmospheric particulate studies,” Appl. Opt. 19, 3389–3395 (1980). [CrossRef] [PubMed]
  16. C. E. Junge, “Our knowledge of the physico-chemistry of aerosols in the undisturbed marine environment,” J. Geophys. Res. 77, 5183–5200 (1972). [CrossRef]
  17. C. E. Junge, E. Robinson, F. L. Ludwig, “A study of aerosols in the Pacific air masses,” J. Appl. Meteorol. 8, 340–347 (1969). [CrossRef]
  18. R. Chesselet, J. Morelli, P. Buat-Menard, “Variations in ionic ratios between reference sea water and marine aerosols,” J. Geophys. Res. 77, 5116–5131 (1972). [CrossRef]
  19. R. Chesselet, M. Fontugne, P. Buat-Ménard, U. Ezat, C. E. Lambert, “The origin of particulate organic carbon in the marine atmosphere as indicated by its stable carbon isotopic composition,” Geophys. Res. Lett. 8, 345–348 (1981). [CrossRef]
  20. O. B. Toon, J. B. Pollack, “A global average model of atmospheric aerosols for radiative transfer calculations,” J. Appl. Meteorol. 15, 225–246 (1976). [CrossRef]
  21. J. L. Gras, G. P. Ayers, “Marine aerosol at southern mid-latitudes,” J. Geophys. Res. 88, 10,661–10,666 (1983). [CrossRef]
  22. T. S. Bates, J. A. Calhoun, P. K. Quinn, “Variations in the methanesulfonate to sulfate molar ratio in submicrometer marine aerosol particles over the South Pacific Ocean,” J. Geophys. Res. 97, 9859–9865 (1992). [CrossRef]
  23. T. Novakov, J. E. Penner, “The effect of anthropogenic sulfate aerosols on marine cloud droplet concentrations,” Nature 365, 823–826 (1992). [CrossRef]
  24. D. K. Woolf, E. C. Monahan, D. E. Spiel, “Quantification of the marine aerosol produced by whitecaps,” in Preprint, Seventh Conference on Ocean-Atmosphere Interaction (American Meteorological Society, Boston, Mass., 1988), pp. 182–185.
  25. E. P. Shettle, R. W. Fenn, Models for the aerosols of the lower atmosphere and the effects of humidity variations on their optical properties, (Air Force Geophysics Laboratory, Hanscomb Air Force Base, Mass., 1979).
  26. A. Mészáros, K. Vissy, “Concentration, size distribution, and chemical nature of atmospheric aerosol particles in remote oceanic areas,” Aerosol Sci. 5, 101–109 (1974). [CrossRef]
  27. M. O. Andreae, “The ocean as a source of atmospheric sulfur compounds,” in The Role of Air-Sea Exchange in Geochemical Cycling, P. Buat-Menard, ed. (Reidel, Dordrecht, The Netherlands, 1986), pp. 331–362. [CrossRef]
  28. R. J. Charlson, J. E. Lovelock, M. O. Andreae, S. G. Warren, “Oceanic phytoplankton, atmospheric sulphur, cloud albedo and climate,” Nature (London) 326, 655–661 (1987).
  29. R. A. Duce, A. H. Woodcock, “Difference in chemical composition of atmospheric sea-salt particles produced in the surf zone and on the open sea in Hawaii,” Tellus 23, 427–435 (1971). [CrossRef]
  30. C. S. Wang, R. L. Street, “Measurements of spray at an air-water interface,” in Dynamics of Atmospheres and Oceans (Elsevier, Amsterdam, 1978), Vol. 2, pp. 141–152. [CrossRef]
  31. M. Komabayashi, “Enrichment of inorganic ions with increasing atomic weight in aerosols, rainwater, and snow in comparison with sea water,” Meteorol. Soc. Jpn. 40, 25–38 (1962).
  32. G. Häanel, “The properties of atmospheric aerosol particles as functions of the relative humidity at thermodynamic equilibrium with the surrounding moist air,” Adv. Geophys. 19, 73–188 (1976). [CrossRef]
  33. E. C. Monahan, C. W. Fairall, K. L. Davidson, P. J. Boyle, “Observed inter-relations between 10 m winds, ocean whitecaps, and marine aerosols,” Q. J. R. Meteorol. Soc. 109, 379–392 (1983). [CrossRef]
  34. V. N. Kapustin, D. S. Covert, “Measurements of the humidification processes of hygroscopic particles,” Appl. Opt. 19, 1349–1352 (1980). [CrossRef] [PubMed]
  35. J. Latham, M. H. Smith, “Effect on global warming of wind-dependent aerosol generation at the ocean surface,” Nature (London) 347, 372–373 (1990).
  36. S. G. Gathman, K. L. Davidson, “The Navy oceanic vertical aerosol model,” (Naval Command, Control and Ocean Surveillance Center, San Diego, Calif., 1993).
  37. G. M. Hale, M. R. Querry, “Optical constants of water in the 200-nm to 200-µm wavelength region,” Appl. Opt. 12, 555–563 (1973). [CrossRef] [PubMed]
  38. F. E. Volz, “Infrared refractive index of atmospheric aerosol substance,” Appl. Opt. 11, 755–759 (1972). [CrossRef] [PubMed]
  39. N. E. Dorsey, Properties of Ordinary Water-Substance in All Its Phases: Water Vapor, Water and All the Ices, Vol. 81 of American Chemical Society Monograph Series (Reinhold, New York, 1940), pp. 332–338.
  40. H. C. van de Hulst, Light Scattering by Small Particles (Wiley, New York, 1957).
  41. C. F. Bohren, D. R. Huffman, Absorption and Scattering of Light by Small Particles (Wiley, New York, 1983).
  42. A. J. Hunt, D. R. Huffman, “A polarization-modulated light scattering instrument for determining liquid aerosol properties,” Jpn. J. Appl. Phys. 14 (Suppl. 14–1), 435–440 (1975).
  43. A. C. Holland, G. Gagne, “The scattering of polarized light by polydisperse systems of irregular particles,” Appl. Opt. 9, 1113–1121 (1970). [CrossRef] [PubMed]
  44. K. J. Voss, E. S. Fry, “Measurement of the Mueller matrix for ocean water,” Appl. Opt. 23, 4427–4439 (1984). [CrossRef] [PubMed]
  45. E. S. Fry, K. J. Voss, “Measurement of the Mueller matrix for phytoplankton,” Limnol. Oceanogr. 30, 1322–1326 (1985). [CrossRef]
  46. M. S. Quinby-Hunt, A. J. Hunt, K. Lofftus, D. B. Shapiro, “Polarized-light scattering studies of marine Chlorella,” Limnol. Oceanogr. 34, 1587–1600, (1989). [CrossRef]
  47. D. R. Huffman, Department of Physics, University of Arizona, Tucson, Ariz., 85721 (personal communication, 1995).
  48. E. S. Fry, G. Kattawar, “Relationships between elements of the Stokes matrix,” Appl. Opt. 20, 2811–2814 (1981). [CrossRef] [PubMed]
  49. G. W. Kattawar, E. S. Fry, “Inequalities between the elements of the Mueller scattering matrix: comments” Appl. Opt. 21, 18 (1982). [CrossRef]
  50. D. Miller, M. S. Quinby-Hunt, A. J. Hunt, “Laboratory studies of the angle and polarization dependent light scattering in sea ice,” Appl. Opt. 36, 1278–1288 (1997). [CrossRef] [PubMed]
  51. D. Miller, M. S. Quinby-Hunt, A. J. Hunt, “A novel bistatic polarization nephelometer for probing scattering through a planar interface,” Rev. Sci. Instrum. 67, 2089–2095 (1997). [CrossRef]
  52. A. J. Hunt, “An experimental investigation of the angular dependence of polarization of light scattered from small particles,” Ph.D. dissertation (University of Arizona, Tucson, Ariz., 1974).
  53. A. J. Hunt, D. R. Huffman, “A new polarization-modulated light scattering instrument,” Rev. Sci. Instrum. 44, 1753–1762 (1973). [CrossRef]
  54. X. Quan, E. S. Fry, “Empirical equation for the index of refraction of seawater,” Appl. Opt. 34, 3477–3480 (1995). [CrossRef] [PubMed]
  55. R. M. Garrels, F. T. Mackenzie, Evolution of Sedimentary Rocks (Norton, New York, 1971), p. 212.
  56. E. T. Arakawa, M. W. Williams, T. Inagaki, “Optical properties of arc-evaporated carbon films between 0.6 and 3.8 eV,” J. Appl. Phys. 48, 3176–3177 (1977). [CrossRef]
  57. A. B. Pluchino, S. S. Goldberg, J. M. Dowling, C. M. Randall, “Refractive-index measurements of single micron-sized carbon particles,” Appl. Opt. 19, 3370–3372 (1980). [CrossRef] [PubMed]
  58. C. E. Batten, “Spectral optical constants of soots from polarized angular reflectance measurements,” Appl. Opt. 24, 1193–1199 (1985). [CrossRef]
  59. F. Parungo, B. Kopcewicz, C. Nagamoto, R. Schnell, P. Sheridan, C. Zhu, J. Harris, “Aerosol particles in the Kuwait oil fire plumes: their morphology, size distribution, chemical composition, transport, and potential effect on climate,” J. Geophys. Res. 97, 15,867–15,882 (1992). [CrossRef]
  60. W. H. Dalzell, A. F. Sarofim, “Optical constants of soot and their application to heat-flux calculations,” J. Heat Transfer 91, 100–104 (1969). [CrossRef]
  61. J. R. Hodkinson, “Refractive index and extinction efficiency factors for carbon,” J. Opt. Soc. Am. 54, 846 (1964). [CrossRef]
  62. V. R. Stull, G. N. Plass, “Emissivity of dispersed carbon particles,” J. Opt. Soc. Am. 50, 121–129 (1960). [CrossRef]

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