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Applied Optics

Applied Optics

APPLICATIONS-CENTERED RESEARCH IN OPTICS

  • Vol. 38, Iss. 9 — Mar. 20, 1999
  • pp: 1418–1422

Minority species detection in aerosols by stimulated anti-Stokes–Raman scattering and external seeding

Victor E. Roman, Jürgen Popp, Mitchell H. Fields, and Wolfgang Kiefer  »View Author Affiliations


Applied Optics, Vol. 38, Issue 9, pp. 1418-1422 (1999)
http://dx.doi.org/10.1364/AO.38.001418


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Abstract

A novel technique applicable to remote sensing has been developed for determination of the chemical composition of microdroplets. Enhancement of stimulated anti-Stokes–Raman scattering (SARS) by external seeding of stimulated Raman scattering (SRS) at the Stokes shift lowers the detection limit of the minority species in multicomponent microdroplets. The technique is most useful in the investigation of microdroplets that contain fluorophores that can obscure the SRS signal. The SARS signal is to the blue of the pump laser and out of the fluorescence region of the fluorophore. Information about majority and minority species in multicomponent microdroplets can be determined from the enhanced SARS signals.

© 1999 Optical Society of America

OCIS Codes
(010.1100) Atmospheric and oceanic optics : Aerosol detection
(190.3970) Nonlinear optics : Microparticle nonlinear optics
(290.5910) Scattering : Scattering, stimulated Raman
(300.6230) Spectroscopy : Spectroscopy, coherent anti-Stokes Raman scattering

History
Original Manuscript: May 26, 1998
Revised Manuscript: August 27, 1998
Published: March 20, 1999

Citation
Victor E. Roman, Jürgen Popp, Mitchell H. Fields, and Wolfgang Kiefer, "Minority species detection in aerosols by stimulated anti-Stokes–Raman scattering and external seeding," Appl. Opt. 38, 1418-1422 (1999)
http://www.opticsinfobase.org/ao/abstract.cfm?URI=ao-38-9-1418

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