A new dye, trans-4-[p-(pyrrolidinyl)styryl]-N-methylpyridinium iodide, has been synthesized, and the two-photon-absorption (TPA), TPA-induced frequency upconversion emission, and two-photon-pumped (TPP) frequency upconverted lasing properties of this new dye were experimentally studied. This new dye has a moderate TPA cross section of σ2 = 5.7 × 10-48 (cm4 s-1)/photon at 1064 nm but exhibits high lasing efficiency. The slope efficiency of the TPP cavity laser with this new dye as the laser medium is 1.6%.
© 2001 Optical Society of America
Original Manuscript: June 25, 2000
Revised Manuscript: December 18, 2000
Published: May 20, 2001
Chun Wang, Xiaomei Wang, Zongshu Shao, Xian Zhao, Guangyong Zhou, Dong Wang, Qi Fang, and Minhua Jiang, "Optical properties of a new two-photon absorbing chromophore," Appl. Opt. 40, 2475-2478 (2001)