${\mathrm{TbAl}}_3({\mathrm{BO}}_3{)}_4$ single crystal was grown from a ${\mathrm{K}}_2{\mathrm{Mo}}_3{\mathrm{O}}_{10}-{\mathrm{B}}_2{\mathrm{O}}_3$ system using the top-seeded high temperature solution method (TSSG), $20\mathrm{mm}\times 9\mathrm{mm}\times 7\mathrm{mm}$ in size. The grown crystal was characterized by x-ray diffraction analysis showing that the crystal has a trigonal structure and the space group is R32 with lattice parameters of $a=b=9.293(13)\AA$ , $c=7.249(6)\AA$ . Faraday rotations of ${\mathrm{TbAl}}_3({\mathrm{BO}}_3{)}_4$ crystal were investigated at room temperature at wavelengths of 532, 633, and 1064 nm. Finally, the Verdet constants were measured at $V=-108.8$ , $-85.7$ , and $-20.8\mathrm{rad}/\mathrm{mT}$ for 532, 633, and 1064 nm, respectively.

© 2011 Optical Society of America

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