Abstract

The third-order susceptibility is expressed as a summation of interfering resonant terms, each involving the phenomenological linewidth of the transition. Correlations of the finite line-width of the laser sources with |<i>X</i>⁽³⁾|² (coherent anti-Stokes Raman spectroscopy) and –<i>X"</i> (stimulated Raman scattering) are performed and closed-form expressions for the theoretical profiles are obtained.

Asymmetric spectral noise correlations in coherent Stokes and anti-Stokes Raman scatterings

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Stimulated Raman scattering and coherent anti-Stokes Raman spectroscopy in high-pressure oxygen

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Raman optical activity by coherent anti-Stokes Raman scattering spectral interferometry

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Vibrational spectroscopy and imaging with non-resonant coherent anti-Stokes Raman scattering: double stimulated Raman scattering scheme

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Spatial-spectral coupling in coherent anti-Stokes Raman scattering microscopy

Aaron M. Barlow, Konstantin Popov, Marco Andreana, Douglas J. Moffatt, Andrew Ridsdale, Aaron D. Slepkov, James L. Harden, Lora Ramunno, and Albert Stolow
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