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Applied Spectroscopy

Applied Spectroscopy

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  • Vol. 52, Iss. 3 — Mar. 1, 1998
  • pp: 380–392

Experimental Studies for a New Family of Infrared FourWave Mixing Spectroscopies

Peter C. Chen, James P. Hamilton, Arne Zilian, Mitchell J. Labuda, and John C. Wright

Applied Spectroscopy, Vol. 52, Issue 3, pp. 380-392 (1998)


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Abstract

Vibrationally enhanced infrared and vibrationally enhanced Raman four-wave mixing spectroscopy are experimentally explored with the use of several model systems. Studies involving a mixture of chlorobenzene, dichlorobenzene, and deuterobenzene were performed to see whether a simultaneous resonance of a combination band could enhance the Raman ring breathing mode. The results show strong interference effects that may be responsible for a suppression of the Raman resonances. Studies were also carried out in systems of chloroform/deuterobenzene and hexane/deuterobenzene. The latter samples showed intensity increases and line-shape changes that are consistent with vibrational enhancement. The discovery of these enhancements form the basis for developing infrared four-wave mixing as a method for extracting new information about molecular vibrations.

Citation
Peter C. Chen, James P. Hamilton, Arne Zilian, Mitchell J. Labuda, and John C. Wright, "Experimental Studies for a New Family of Infrared FourWave Mixing Spectroscopies," Appl. Spectrosc. 52, 380-392 (1998)
http://www.opticsinfobase.org/as/abstract.cfm?URI=as-52-3-380

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