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Chinese Optics Letters

Chinese Optics Letters

| PUBLISHED MONTHLY BY CHINESE LASER PRESS AND DISTRIBUTED BY OSA

  • Editor: Zhizhan Xu
  • Vol. 10, Iss. 11 — Nov. 1, 2012
  • pp: 111601–111601

Ultrafast third-order optical nonlinearities in DMSO

Degui Kong, Guanghong Ao, Yachen Gao, Qing Chang, and Hong'an Ye  »View Author Affiliations


Chinese Optics Letters, Vol. 10, Issue 11, pp. 111601-111601 (2012)


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Abstract

The third-order optical nonlinearities of dimethyl sulfoxide (DMSO) are investigated using the optical Kerr effect (OKE) and Z-scan techniques with femtosecond pulses. We are able to fit the OKE signal theoretically by convolving the autocorrelation of the incident pulse intensity profile with the impulse responses of the samples, illustrating the instantaneous nonlinear response of DMSO. We verify that the purely electronic cloud distortion causes the observed signal for DMSO. The Z-scan technique is used to estimate the third-order susceptibility of DMSO, which is about a quarter of that for CS2 and mainly comes from the nonlinear refraction with an intensity of less than 140 GW/cm2.

© 2012 Chinese Optics Letters

OCIS Codes
(160.4670) Materials : Optical materials
(190.3270) Nonlinear optics : Kerr effect

ToC Category:
Materials

Citation
Degui Kong, Guanghong Ao, Yachen Gao, Qing Chang, and Hong'an Ye, "Ultrafast third-order optical nonlinearities in DMSO," Chin. Opt. Lett. 10, 111601-111601 (2012)
http://www.opticsinfobase.org/col/abstract.cfm?URI=col-10-11-111601


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