Beam-foil study of sulfur between 500 and 1200 Å

P. D. Dumont; H. P. Garnir; Y. Baudinet-Robinet

doi:10.1364/JOSA.68.000825

Journal of the Optical Society of America
Vol. 68,
Issue 6,
pp. 825-829
(1978)
•https://doi.org/10.1364/JOSA.68.000825

Beam-foil study of sulfur between 500 and 1200 Å

P. D. Dumont, H. P. Garnir, and Y. Baudinet-Robinet

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P. D. Dumont, H. P. Garnir, and Y. Baudinet-Robinet, "Beam-foil study of sulfur between 500 and 1200 Å," J. Opt. Soc. Am. 68, 825-829 (1978)

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Abstract

Beam-foil spectra of sulfur have been studied between 500 and 1200 Å. Lifetime measurements have been performed for 33 levels in S iii – S vi (first measurements for 14 levels.) Our lifetime results are compared with other experimental and theoretical values where possible. Three new classifications are proposed in S vi.

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Wavelength (Å)	Transition
627.9 ± 0.2	$4 s {{}^{2}S}_{1 / 2} - 5 p {{}^{2}P}_{3 / 2}^{0}$
692.5 ± 0.2	$4 p^{2} P_{3 / 2}^{0} - 5 d^{2} D_{3 / 2, 5 / 2}$
1000.3 ± 0.2	4d ²D–5f ²F⁰

Wavelength (Å)	Probable ionization stage	Lifetime of upper term (ns)	Lifetime of cascades (ns)	R(0)^a
577.7 ± 0.2	v (or vi)	0.096 ± 0.012	0.5 ± 0.1, ≃5	0.15
610.7 ± 0.2	iv (or v)	0.12 ± 0.02	2.7 ± 0.4	0.09
611.7 ± 0.2	iv (or v)	0.13 ± 0.02	2.6 ± 0.4	0.12
625.9 ± 0.2	iv (or v)	0.11 ± 0.01	3.5 ± 1.1	0.06
672.2 ± 0.2	vi (or vii)	0.033 ± 0.01	3.1 ± 0.2	0.06
672.7 ± 0.2	iv (or v)	0.068 ± 0.016	0.30 ± 0.04, 5.7 ± 0.3	0.5
675.5 ± 0.2	iv (or v)	0.065 ± 0.014	0.32 ± 0.02, 4.0 ± 0.5	0.5
677.4 ± 0.2^b	vii (or viii)	0.24 ± 0.01	⋯	⋯
710.9 ± 0.2	iii	0.11 ± 0.01	3.1 ± 1.0	0.05
716.8 ± 0.2	v	0.130 ± 0.005	1.7 ± 0.2	0.09
769.8 ± 0.2	vii (or vi)	0.35 ± 0.02	3.3 ± 0.5	0.05
781.3 ± 0.2	vii (or vi)	0.24 ± 0.01	9.1 ± 2.0	0.06
887.7 ± 0.2	vii (or vi)	0.66 ± 0.10	≃5	0.07
906.0 ± 0.2^b	vi	≃3	⋯	⋯
924.2 ± 0.2	vii (or viii)	0.63 ± 0.06	0.06, ≃5	≃5

Ion	Transition	Wavelength (Å)	This work		Theory		R(0)^a
S iii	$3 p^{2} {{}^{3}P}_{1} - 3 d {{}^{3}D}_{1}^{0}$	679.1	0.11 ± 0.02		⋯	0.6 ± 0.2, 3.4 ± 0.8	0.13
	$3 p^{2} {{}^{3}P}_{2} - 3 d {{}^{3}D}_{2, 3}^{0}$	680.8	0.09 ± 0.02	0.12^b	⋯	0.8 ± 0.1, 6.0 ± 0.8	0.17
	$3 p^{2} {{}^{3}P}_{1, 2} - 4 s {{}^{3}P}_{0, 2}^{0}$	683.3	0.09 ± 0.01	⋯	⋯	0.38 ± 0.06, 4.4 ± 0.4	0.2
	$3 p^{2} {{}^{3}P}_{1} - 3 d {{}^{3}P}_{2, 0}^{0}$	700.2	0.12 ± 0.01	⋯	⋯	2.5 ± 0.3	0.05
	$3 p^{2} {{}^{3}P}_{2} - 3 d {{}^{3}P}_{2, 1}^{0}$	702.8	0.12 ± 0.02	⋯	⋯	2.4 ± 0.4	0.05
S iv	3p^{2 4}P–3d ⁴D⁰	655.6	0.099 ± 0.006	0.117^b	⋯	0.41 ± 0.07, 5.4 ± 0.4	0.2
	$3 p {{}^{2}P}_{1 / 2}^{0} - 3 d {{}^{2}D}_{3 / 2}$	657.3	0.140 ± 0.008	⋯	0.09^d	3.3 ± 0.2	0.08
	$3 p {{}^{2}P}_{3 / 2}^{0} - 3 d {{}^{2}D}_{5 / 2}$	661.4	0.139 ± 0.009	0.12^b		2.0 ± 0.2	0.08
	$3 p^{2} {{}^{4}P}_{5 / 2} - 3 d {{}^{4}P}_{5 / 2}^{0}$	666.1	0.19 ± 0.01	⋯	⋯	2.8 ± 0.3, >500	0.1
	$3 p {{}^{2}P}_{1 / 2}^{0} - 3 p^{2} {{}^{2}P}_{1 / 2}$	748.4	0.176 ± 0.009	0.15^b	⋯	3.3 ± 0.7	0.04
	$3 p {{}^{2}P}_{3 / 2}^{0} - 3 p^{2} {{}^{2}P}_{3 / 2}$	750.2
	$3 p {{}^{2}P}_{3 / 2}^{0} - 3 p^{2} {{}^{2}P}_{1 / 2}$	753.8
	$3 p {{}^{2}P}_{3 / 2}^{0} - 3 p^{2} {{}^{2}S}_{1 / 2}$	816.0	0.428 ± 0.008	0.216^b	⋯	3.6 ± 1.6	0.03
S v	$3 p {{}^{3}P}_{0}^{0} - 3 d {{}^{3}D}_{1}$	658.3	0.18 ± 0.02	⋯	0.155,^e 0.16^f	≃1, ≳10	0.2
	$3 p {{}^{3}P}_{1}^{0} - 3 d {{}^{3}D}_{2}$	659.9	0.209 ± 0.009	⋯
	$3 p {{}^{3}P}_{2}^{0} - 3 d {{}^{3}D}_{3}$	663.2	0.200 ± 0.008	0.17,^b (1.7)^g
	$3 p^{2} {{}^{3}P}_{0} - 3 d {{}^{3}D}_{1}^{0}$	676.2	0.10 ± 0.01	⋯	0.09^e,^f	0.5 ± 0.1, 5 ± 3	0.1
	$3 p^{2} {{}^{3}P}_{2} - 3 d {{}^{3}D}_{2}^{0}$	680.9	0.13 ± 0.01	⋯	0.09^e,^f	0.8 ± 0.2	0.08
	$3 p^{2} {{}^{3}P}_{2} - 3 d {{}^{3}P}_{2}^{0}$	693.5	0.14 ± 0.02	0.26^b	0.14,^e 0.13^f	0.7 ± 0.1	0.2
	$3 p {{}^{1}P}_{1}^{0} - 3 d {{}^{1}D}_{2}$	696.5^h	0.098 ± 0.010	0.13^b	0.093,ⁱ 0.088^f	0.5 ± 0.1, 6 ± 2	≃0.2
					0.105^e
	3p^{2 1}D–3d ¹D⁰	742.2^c	0.27 ± 0.01	⋯	0.23,^e 0.21^f	2.2 ± 0.4	0.03
	$3 s^{2} {{}^{1}S}_{0} - 3 p {{}^{1}P}_{1}^{0}$	786.5	0.28 ± 0.01	0.263^b, 0.16,^j (1.14)^g	0.19,^k 0.20^e,^f	0.05 ± 0.02, 4.4 ± 0.3	≃5
	$3 p {{}^{3}P}_{1}^{0} - 3 p^{2} {{}^{3}P}_{2}$	849.2	0.28 ± 0.03	0.32,^b (0.75)^g	0.24^e,^f	0.08 ± 0.02, 2.3 ± 0.4	≃1
	$3 p {{}^{3}P}_{2}^{0} - 3 p^{2} {{}^{3}P}_{2}$	854.8	0.26 ± 0.02
	$3 p {{}^{3}P}_{1}^{0} - 3 p^{2} {{}^{3}P}_{0}$	857.9	0.28 ± 0.03
	$3 p {{}^{3}P}_{2}^{0} - 3 p^{2} {{}^{3}P}_{1}$	860.5	0.28 ± 0.03
	$3 d {{}^{3}D}_{1, 2, 3} - 4 p {{}^{3}P}_{2}^{0}$	873.0^l	0.79 ± 0.05	⋯	0.64^f	0.18 ±0.08, ≳10	≃1
	$3 d {{}^{3}D}_{3} - 3 d {{}^{3}D}_{3}^{0}$	883.6	0.11 ± 0.01	⋯	0.09^e,^f	1.4 ± 0.6	0.08
	$3 d {{}^{3}D}_{3} - 3 d {{}^{3}F}_{4}^{0}$	1122.0^m	1.2 ± 0.2	(1.9)^g	1.0^e	7 ± 3	0.1
S vi	$3 d {{}^{2}D}_{5 / 2} - 4 p {{}^{2}P}_{3 / 2}^{0}$	648.6	0.28 ± 0.01	⋯	0.15,^k 0.14,ⁿ 0.18^o	3.1 ± 0.4	0.06
	$3 d {{}^{2}D}_{3 / 2} - 4 p {{}^{2}P}_{1 / 2}^{0}$	650.4	0.26 ± 0.02	⋯	0.15,^k 0.14,ⁿ 0.18^o	3.1 ± 0.4	0.06
	$3 p {{}^{2}P}_{1 / 2}^{0} - 3 d {{}^{2}D}_{3 / 2}$	706.5	0.23 ± 0.01			1.0 ± 0.3, ≃8	0.08
				0.25,^b (1.0)^g	0.20,^e 0.24,ⁿ 0.19^o
	$3 p {{}^{2}P}_{3 / 2}^{0} - 3 d {{}^{2}D}_{5 / 2, 3 / 2}$	712.7	0.25 ± 0.01			1.0 ± 0.2, ≃7	0.06
	4f ²F⁰–6g ²G	725.8^c	0.21 ± 0.04	(1.09)^g,^p	⋯	≃ 2, ≳ 20	≃0.2
	$3 s {{}^{2}S}_{1 / 2} - 3 p {{}^{2}P}_{3 / 2}^{0}$	933.4	0.65 ± 0.03	0.71,^b 0.74^j	0.61,^e 0.69,ⁿ 0.59^o, 0.60^q	0.24 ± 0.02, 4.7 ± 0.6	≃2
	$3 s {{}^{2}S}_{1 / 2} - 3 p {{}^{2}P}_{1 / 2}^{0}$	944.5	0.67 ± 0.03	0.69^b	0.63,^e 0.72,ⁿ 0.61^o, 0.62^q	0.22 ± 0.02, 4.9 ± 0.8	≃2
	4d ²D–5f ²F⁰	1000.3^s	0.13 ± 0.02	⋯	0.095^o	0.7 ±0.3, ≃10	≃2.5
	4f ²F⁰–5g ²G	1117.9	0.24 ± 0.04	(3.1)^g	0.18^r	1.6 ± 0.4, ≃25	0.36

Wavelength (Å)	Transition
627.9 ± 0.2	$4 s {{}^{2}S}_{1 / 2} - 5 p {{}^{2}P}_{3 / 2}^{0}$
692.5 ± 0.2	$4 p^{2} P_{3 / 2}^{0} - 5 d^{2} D_{3 / 2, 5 / 2}$
1000.3 ± 0.2	4d ²D–5f ²F⁰

Wavelength (Å)	Probable ionization stage	Lifetime of upper term (ns)	Lifetime of cascades (ns)	R(0)^a
577.7 ± 0.2	v (or vi)	0.096 ± 0.012	0.5 ± 0.1, ≃5	0.15
610.7 ± 0.2	iv (or v)	0.12 ± 0.02	2.7 ± 0.4	0.09
611.7 ± 0.2	iv (or v)	0.13 ± 0.02	2.6 ± 0.4	0.12
625.9 ± 0.2	iv (or v)	0.11 ± 0.01	3.5 ± 1.1	0.06
672.2 ± 0.2	vi (or vii)	0.033 ± 0.01	3.1 ± 0.2	0.06
672.7 ± 0.2	iv (or v)	0.068 ± 0.016	0.30 ± 0.04, 5.7 ± 0.3	0.5
675.5 ± 0.2	iv (or v)	0.065 ± 0.014	0.32 ± 0.02, 4.0 ± 0.5	0.5
677.4 ± 0.2^b	vii (or viii)	0.24 ± 0.01	⋯	⋯
710.9 ± 0.2	iii	0.11 ± 0.01	3.1 ± 1.0	0.05
716.8 ± 0.2	v	0.130 ± 0.005	1.7 ± 0.2	0.09
769.8 ± 0.2	vii (or vi)	0.35 ± 0.02	3.3 ± 0.5	0.05
781.3 ± 0.2	vii (or vi)	0.24 ± 0.01	9.1 ± 2.0	0.06
887.7 ± 0.2	vii (or vi)	0.66 ± 0.10	≃5	0.07
906.0 ± 0.2^b	vi	≃3	⋯	⋯
924.2 ± 0.2	vii (or viii)	0.63 ± 0.06	0.06, ≃5	≃5

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Journal of the Optical Society of America