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Journal of the Optical Society of America A

Journal of the Optical Society of America A


  • Vol. 15, Iss. 8 — Aug. 1, 1998
  • pp: 2066–2077

Diffusive wave illumination: light-scattering study of colloidal dynamics in opaque media

I. Flammer, G. Bucher, and J. Rička  »View Author Affiliations

JOSA A, Vol. 15, Issue 8, pp. 2066-2077 (1998)

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Microscopic movements of latex particles in the water-filled voids of a glass bead packing are investigated with a variant of dynamic light-scattering, diffusive wave illumination. We are able to measure simultaneously diffusive and convective motion of the scatterers within the pore spaces of the completely opaque medium. The influence of increased seepage velocity on the diffusion coefficient and on the speed distribution of the particles is studied. We find an exponential distribution of the convective speed. From the average speed we determine the tortuosity of the packing. Using this investigation system as an illustration, we address the methodological aspects of diffusive wave illumination and discuss its possibilities and limitations: (1) the possibility of tuning the amount of local oscillator mixed to the dynamic signal, (2) the inclusion of residual dynamics of the porous medium into the fitting model, and (3) a study of the influence of increased particle concentration on the signal correlation function.

© 1998 Optical Society of America

OCIS Codes
(280.2490) Remote sensing and sensors : Flow diagnostics
(290.4210) Scattering : Multiple scattering
(290.7050) Scattering : Turbid media

Original Manuscript: August 29, 1997
Revised Manuscript: January 14, 1998
Manuscript Accepted: March 18, 1998
Published: August 1, 1998

I. Flammer, G. Bucher, and J. Rička, "Diffusive wave illumination: light-scattering study of colloidal dynamics in opaque media," J. Opt. Soc. Am. A 15, 2066-2077 (1998)

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  1. P. C. Carman, “Fluid flow through granular beds,” Trans. Inst. Chem. Eng. 15, 150–156 (1937).
  2. E. Charlaix, J. P. Hulin, T. J. Plona, “Experimental study of tracer dispersion in sintered glass porous materials of variable compaction,” Phys. Fluids 30, 1690–1698 (1987). [CrossRef]
  3. Y. D. Yan, M. Borkovec, H. Sticher, “Deposition and release of colloidal particles in porous media,” Prog. Colloid Polym. Sci. 98, 132–135 (1995). [CrossRef]
  4. W. Johnston, A. Dybbs, “Measurement of fluid velocity inside porous media with a laser anemometer,” Phys. Fluids 18, 913–914 (1975). [CrossRef]
  5. M. T. Bishop, K. H. Langley, F. E. Karasz, “Diffusion of a flexible polymer in a random porous material,” Phys. Rev. Lett. 57, 1741–1744 (1986). [CrossRef] [PubMed]
  6. M. T. Bishop, K. H. Langley, F. E. Karasz, “Dynamic light-scattering studies of polymer diffusion in porous materials: linear polystyrene in porous glass,” Macromolecules 22, 1220–1231 (1989). [CrossRef]
  7. R. Bonner, R. Nossal, “Model for laser Doppler measurements of blood flow in tissue,” Appl. Opt. 20, 2097–2107 (1981). [CrossRef] [PubMed]
  8. D. J. Pine, D. A. Weitz, G. Maret, P. E. Wolf, E. Herbolzheimer, P. M. Chaikin, in Classical Wave Localisation, P. Sheng, ed. (World Scientific, London, 1989).
  9. J. Rička, “Brownian dynamics in strongly scattering porous media: dynamic light scattering with single-mode matching,” Makromol. Chem. Macromol. Symp. 79, 45–55 (1994). [CrossRef]
  10. J. Rička, I. Flammer, W. Leutz, “Single-mode DLS: colloids in opaque porous media,” Prog. Colloid Polym. Sci. 104, 49–58 (1997).
  11. I. Flammer, J. Rička, “Dynamic light scattering with single-mode receivers: partial heterodyning regime,” Appl. Opt. 36, 7508–7517 (1997). [CrossRef]
  12. J. Rička, “Dynamic light scattering with single-mode and multimode receivers,” Appl. Opt. 32, 2860–2875 (1993). [CrossRef] [PubMed]
  13. Recent developments on DWS and related methods are found in the feature issue on diffusing photons in turbid media, J. Opt. Soc. Am. A 14, 136–342 (1997).
  14. G. Maret, P. Wolf, “Multiple light scattering from disordered media: the effect of Brownian motion on scatterers,” Z. Phys. B 65, 409–413 (1987). [CrossRef]
  15. D. J. Pine, D. A. Weitz, J. X. Zhu, E. Herbolzheimer, “Diffusing-wave spectroscopy: dynamic light scattering in the multiple scattering limit,” J. Phys. (France) 51, 2101–2127 (1990). [CrossRef]
  16. P. N. Pusey, “Dynamic light scattering by non-ergodic media,” Physica A 157, 705–741 (1989). [CrossRef]
  17. K. Schätzel, “Dead time correction of photon correlation functions,” Appl. Phys. B 41, 95–102 (1986). [CrossRef]
  18. F. T. Arecchi, M. Corti, V. Degiorgio, S. Donati, “Measurements of light intensity correlations in the subnanosecond region by photomultipliers,” Opt. Commun. 3, 284–288 (1971). [CrossRef]
  19. H. Hulst, Light Scattering by Small Particles (Wiley, New York, 1957).
  20. R. T. Foister, T. G. van de Ven, “Diffusion of Brownian particles in shear flows,” J. Fluid Mech. 96, 105–132 (1980). [CrossRef]
  21. T. G. M. V. de Ven, Colloidal Hydrodynamics (Academic, London, 1989).
  22. N. G. van Kampen, Stochastic Processes in Physics and Chemistry (North-Holland, Amsterdam, 1981).
  23. H. S. Carslaw, J. C. Jaeger, Conduction of Heat in Solids (Oxford Science Publications, Oxford, UK, 1959), Chap. XIV.
  24. W. Leutz, J. Rička, “On light propagation through glass bead packings,” Opt. Commun. 126, 260–268 (1996). [CrossRef]
  25. D. E. Koppel, “Analysis of macromolecular polydispersity in intensity correlation spectroscopy: the method of cumulants,” J. Chem. Phys. 57, 4814–4820 (1972). [CrossRef]
  26. L. R. Snyder, J. J. Kirkland, Introduction to Modern Liquid Chromatography (Wiley, New York, 1979).
  27. J. Bear, Dynamics of Fluids in Porous Media (Dover, New York, 1988).
  28. P. D. Kaplan, M. H. Kao, A. G. Yodh, D. J. Pine, “Geometric constraints for the design of diffusing-wave spectroscopy experiments,” Appl. Opt. 32, 3828–3836 (1993). [CrossRef] [PubMed]
  29. Y. E. Kutsovsky, L. E. Scriven, H. T. Davis, B. E. Hammer, “NMR imaging of velocity profiles and velocity distribution in bead packs,” Phys. Fluids 8, 863–871 (1996). [CrossRef]
  30. L. Lebon, L. Oger, J. Leblond, J. P. Hulin, N. S. Martys, L. M. Schwartz, “Pulsed gradient NMR measurements and numerical simulation of flow velocity distribution in sphere packing,” Phys. Fluids 8, 293–301 (1996). [CrossRef]

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