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Journal of the Optical Society of America B

Journal of the Optical Society of America B


  • Editor: Henry Van Driel
  • Vol. 26, Iss. 4 — Apr. 1, 2009
  • pp: 572–580

Ultrafast nuclear spin polarization for isotopes with large nuclear spin

Takashi Nakajima  »View Author Affiliations

JOSA B, Vol. 26, Issue 4, pp. 572-580 (2009)

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We theoretically investigate the temporal dynamics of nuclear spin induced by short laser pulses. To realize ultrafast nuclear spin polarization, we coherently excite the hyperfine manifolds and let it evolve in time. An appropriate choice of the state with large hyperfine splittings allows us to realize ultrafast nuclear spin polarization. As specific examples, we consider the various isotopes of Mg and Ca with different values of nuclear spin ( 1 2 , 3 2 , 5 2 , and 7 2 ) and show that 89%, 76%, 49%, and 36% of nuclear spin polarization can be achieved, respectively, within a few nanoseconds, which is at least 2 to 3 orders of magnitude shorter than the time needed for any known optical methods. Because of its ultrafast nature, our scheme would be very effective not only for stable nuclei but also unstable nuclei with a lifetime as short as 1 μ s .

© 2009 Optical Society of America

OCIS Codes
(020.4180) Atomic and molecular physics : Multiphoton processes
(270.1670) Quantum optics : Coherent optical effects
(300.6240) Spectroscopy : Spectroscopy, coherent transient

ToC Category:
Atomic and Molecular Physics

Original Manuscript: October 17, 2008
Revised Manuscript: January 23, 2009
Manuscript Accepted: January 26, 2009
Published: March 3, 2009

Takashi Nakajima, "Ultrafast nuclear spin polarization for isotopes with large nuclear spin," J. Opt. Soc. Am. B 26, 572-580 (2009)

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  1. J. Kessler, Polarized Electrons, 2nd Ed., (Springer-Verlag, 1985).
  2. T. Maruyama, E. L. Garwin, R. Prepost, G. H. Zapalac, J. S. Smith, and J. D. Walker, “Observation of strain-enhanced electron-spin polarization in photoemission from InGaAs,” Phys. Rev. Lett. 66, 2376-2379 (1991). [CrossRef] [PubMed]
  3. T. Nakanishi, H. Aoyagi, H. Horinaka, Y. Kamiya, T. Kato, S. Nakamura, T. Saka, and M. Tsubata, “Large enhancement of spin polarization observed by photoelectrons from a strained GaAs layer,” Phys. Lett. A 158, 345-349 (1991). [CrossRef]
  4. D. Fick, G. Grawert, and I. M. Turkiewicz, “Nuclear physics with polarized heavy ions,” Phys. Rep. 214, 1-111 (1992). [CrossRef]
  5. N. B. Delone, B. A. Zon, and M. V. Fedorov, “Polarization of nuclei in resonance ionization of atoms,” Sov. Phys. JETP 49, 255 (1979).
  6. J. T. Cusma and L. W. Anderson, “Polarization of an atomic sodium beam by laser optical pumping,” Phys. Rev. A 28, 1195-1197 (1983). [CrossRef]
  7. G. D. Cates, D. R. Benton, M. Gatzke, W. Happer, K. C. Hasson, and N. R. Newbury, “Laser production of large nuclear-spin polarization in frozen xenon,” Phys. Rev. Lett. 65, 2591-2594 (1990). [CrossRef] [PubMed]
  8. H. Reich and H. J. Jänsch, “Nuclear spin polarized alkali beams (Na,Li): Optical pumping with electro-optically modulated laser beam,” Nucl. Instrum. Methods Phys. Res. A 288, 349-353 (1990). [CrossRef]
  9. A. N. Zelenskii, K. Jayamanna, C. D. P. Levy, M. McDonald, R. Ruegg, and P. W. Schmor, “Optimization studies of proton polarization in the TRIUMF optically pumped polarized H− ion source,” Nucl. Instrum. Methods Phys. Res. A 334, 285-293 (1993). [CrossRef]
  10. C. D. P. Levy, R. Baartman, J. A. Behr, R. F. Kiefl, M. Pearson, R. Poutissou, A. Hatakeyama, and Y. Hirayama, “The collinear laser beam line at ISAC,” Nucl. Phys. A 746, 206C-209C (2004). [CrossRef]
  11. T. Nakajima and N. Yonekura, “Electron spin-polarized alkaline-earth ions produced by multiphoton ionization,” J. Chem. Phys. 117, 2112-2119 (2002). [CrossRef]
  12. T. Nakajima, N. Yonekura, Y. Matsuo, T. Kobayashi, and Y. Fukuyama, “Simultaneous production of spin-polarized ions/electrons based on two-photon ionization of laser-ablated metallic atoms,” Appl. Phys. Lett. 83, 2103-2105 (2003). [CrossRef]
  13. N. Yonekura, T. Nakajima, Y. Matsuo, T. Kobayashi, and Y. Fukuyama, “Electron-spin polarization of photoions produced through photoionization from the laser-excited triplet state of Sr,” J. Chem. Phys. 120, 1806-1812 (2004). [CrossRef] [PubMed]
  14. E. Sokell, S. Zamith, M. A. Bouchene, and B. Girard, “Polarization-dependent pump-probe studies in atomic fine-structure levels: towards the production of spin-polarized electrons,” J. Phys. B 33, 2005-2015 (2000). [CrossRef]
  15. M. A. Bouchene, S. Zamith, and B. Girard, “Spin-polarized electrons produced by a sequence of two femtosecond pulses. Calculation of differential and global polarization rates,” J. Phys. B 34, 1497-1512 (2001). [CrossRef]
  16. T. Nakajima, “Control of the spin-polarization of photoelectrons/photoions using short laser pulses,” Appl. Phys. Lett. 84, 3786-3788 (2004). [CrossRef]
  17. T. Nakajima, “Effects of laser intensity and applied electric field on coherent control of spin polarization by short laser pulses,” Appl. Phys. Lett. 88, 111105 (2006). [CrossRef]
  18. T. Nakajima, Y. Matsuo, and T. Kobayashi, “All-optical control and direct detection of ultrafast spin polarization in a multi-valence-electron system,” Phys. Rev. A 77, 063404 (2008). [CrossRef]
  19. D. J. Tannor and S. A. Rice, “Control of selectivity of chemical-reaction via control of wave packet evolution,” J. Chem. Phys. 83, 5013-5018 (1985). [CrossRef]
  20. H. J. Andra, H. J. Plohn, A. Gaupp, and R. Frohling, “Nuclear-spin polarization produced by ion-beam-surface-interaction, its optical detection and use in an atomic quantum-beat experiment,” Z. Phys. A 281, 15-20 (1977). [CrossRef]
  21. C. Fabre, M. Gross, and S. Haroche, “Determination by quantum beat spectroscopy of fine-structure intervals in a series of highly excited sodium D states,” Opt. Commun. 13, 393 (1975). [CrossRef]
  22. J. S. Deech, R. Luypaert, and G. W. Series, “Determination of lifetimes and hyperfine structures of 8, 9 and 10 D3/22 states of Cs133 by quantum-beat spectroscopy,” J. Phys. B 8, 1406-1414 (1975). [CrossRef]
  23. T. Nakajima, “Investigation of ultrafast nuclear spin polarization induced by short laser pulses,” Phys. Rev. Lett. 99, 024801 (2007). [CrossRef] [PubMed]
  24. M. E. Hayden and E. W. Otten, “Comment on 'Investigation of ultrafast nuclear spin polarization induced by short laser pulses',” Phys. Rev. Lett. 101, 189501 (2008). [CrossRef] [PubMed]
  25. T. Nakajima, “Nakajima replies,” Phys. Rev. Lett. 101, 189502 (2008). [CrossRef]
  26. R. D. Cowan, The Theory of Atomic Structure and Spectra, (U. California Press, 1981).
  27. A. Lurio, “Hyerpfine structure of the P3 states of Zn67 and Mg25,” Phys. Rev. 126, 1768-1773 (1962). [CrossRef]
  28. G. Olsson and S. Salomonson, “Analysis of the hyperfine structure of the 4s4p configuration in Ca and the nuclear quadrupole moment of Ca43,” Z. Phys. A 307, 99-107 (1982). [CrossRef]
  29. A. Mortensen, J. J. T. Lindballe, I. S. Jensen, P. Staanum, D. Voigt, and M. Drewsen, “Isotope shifts of the 4s2S01-->4s5P11 transition and hyperfine splitting of the 4s5pP11 state in calcium,” Phys. Rev. A 69, 042502 (2004). [CrossRef]
  30. T. Nakajima and G. Buica, “Above-threshold ionization of Mg by linearly and circularly polarized laser pulses: Origin of the subpeaks in the photoelectron energy spectra,” Phys. Rev. A 74, 023411 (2006). [CrossRef]

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