Abstract
We use a quantum mechanical approach to derive a set of linear and nonlinear quantum conductivity coefficients for metal–insulator–metal structures with nanometer sized gaps. The immediate proximity of metallic objects generates a tunneling AC current density that endows the gap region with additional linear and nonlinear coefficients that in turn trigger linear and nonlinear absorption, and second- and third-harmonic generation. For example, a vacuum gap approximately 0.8 nm thick displays an effective for adjacent objects composed of dissimilar metals and an effective for either similar or dissimilar metals, increasing exponentially for smaller gaps. Field localization inside the gap ensures that harmonic generation arising from the gap region overwhelms intrinsic metal second- and third-order nonlinearities.
© 2014 Optical Society of America
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