OSA's Digital Library

Journal of the Optical Society of America B

Journal of the Optical Society of America B

| OPTICAL PHYSICS

  • Vol. 17, Iss. 12 — Dec. 1, 2000
  • pp: 2032–2036

Polarization and angle dependence for hyper-Rayleigh scattering from local and nonlocal modes of isotropic fluids

David P. Shelton  »View Author Affiliations


JOSA B, Vol. 17, Issue 12, pp. 2032-2036 (2000)
http://dx.doi.org/10.1364/JOSAB.17.002032


View Full Text Article

Enhanced HTML    Acrobat PDF (133 KB)





Browse Journals / Lookup Meetings

Browse by Journal and Year


   


Lookup Conference Papers

Close Browse Journals / Lookup Meetings

Article Tools

Share
Citations

Abstract

Collective modes of molecular motion result in long-range correlations between molecules. Orientation correlations between the molecules of an isotropic fluid owing to polar collective modes result in hyper-Rayleigh scattering with distinctive polarization and angle dependence. The polarization and angle dependence for hyper-Rayleigh scattering from polar transverse-optical and longitudinal-optical nonlocal modes, and for dipolar and quadrupolar hyper-Raleigh scattering from local modes, is calculated and compared.

© 2000 Optical Society of America

OCIS Codes
(190.4410) Nonlinear optics : Nonlinear optics, parametric processes
(190.4710) Nonlinear optics : Optical nonlinearities in organic materials
(190.4720) Nonlinear optics : Optical nonlinearities of condensed matter

Citation
David P. Shelton, "Polarization and angle dependence for hyper-Rayleigh scattering from local and nonlocal modes of isotropic fluids," J. Opt. Soc. Am. B 17, 2032-2036 (2000)
http://www.opticsinfobase.org/josab/abstract.cfm?URI=josab-17-12-2032


Sort:  Author  |  Year  |  Journal  |  Reset  

References

  1. K. Clays and A. Persoons, “Hyper-Rayleigh scattering in solution,” Phys. Rev. Lett. 66, 2980–2983 (1991). [CrossRef] [PubMed]
  2. K. Clays, A. Persoons, and L. de Maeyer, “Hyper-Rayleigh scattering in solution,” in Modern Nonlinear Optics, I. Prigogine and S. A. Rice, eds., Advances in Chemical Physics (Wiley, New York, 1994), Vol. 85, Pt. 3, pp. 455–498.
  3. G. J. T. Heesink, A. G. T. Ruiter, N. F. van Hulst, and B. Bolger, “Determination of hyperpolarizability tensor components by depolarized hyper Rayleigh scattering,” Phys. Rev. Lett. 71, 999–1002 (1993). [CrossRef] [PubMed]
  4. P. Kaatz and D. P. Shelton, “Spectral measurements of hyper-Rayleigh scattering,” Rev. Sci. Instrum. 67, 1438–1444 (1996). [CrossRef]
  5. D. Morrison, R. G. Denning, W. M. Laidlaw, and M. A. Stammers, “Measurement of first hyperpolarizabilities by hyper-Rayleigh scattering,” Rev. Sci. Instrum. 67, 1445–1453 (1996). [CrossRef]
  6. M. Kauranen and A. Persoons, “Theory of polarization measurements of second-order nonlinear light scattering,” J. Chem. Phys. 104, 3445–3456 (1996). [CrossRef]
  7. S. F. Hubbard, R. G. Petschek, K. D. Singer, N. D’Sidocky, C. Hudson, L. C. Chien, C. C. Henderson, and P. A. Cahill, “Measurements of Kleinman-disallowed hyperpolarizability in conjugated chiral molecules,” J. Opt. Soc. Am. B 15, 289–301 (1998). [CrossRef]
  8. R. W. Terhune, P. D. Maker, and C. M. Savage, “Measurements of nonlinear light scattering,” Phys. Rev. Lett. 14, 681–684 (1965). [CrossRef]
  9. R. Bersohn, Y. H. Pao, and H. L. Frisch, “Double-quantum light scattering by molecules,” J. Chem. Phys. 45, 3184–3198 (1966). [CrossRef]
  10. D. L. Weinberg, “Temperature dependence, orientation correlation, and molecular fields in second-harmonic light scattering from liquids and gases,” J. Chem. Phys. 47, 1307–1313 (1967). [CrossRef]
  11. P. D. Maker, “Spectral broadening of elastic second-harmonic light scattering in liquids,” Phys. Rev. A 1, 923–951 (1970). [CrossRef]
  12. D. P. Shelton and P. Kaatz, “Librons observed in liquid acetonitrile by hyper-Rayleigh scattering,” Phys. Rev. Lett. 84, 1224–1227 (2000). [CrossRef] [PubMed]
  13. D. P. Shelton, “Collective molecular rotation in water and other simple liquids,” Chem. Phys. Lett. 325, 513–516 (2000). [CrossRef]
  14. S. Kielich and M. Kozierowski, “Symmetric and antisymmetric second-harmonic elastic light scattering and its angular dependences,” Acta Phys. Pol. A 45, 231–251 (1974).
  15. K. Altmann and G. Strey, “The hyper-Raman effect in molecular gases,” J. Raman Spectrosc. 12, 1–15 (1982). [CrossRef]
  16. S. Kielich, “Multi-photon scattering molecular spectroscopy,” Progress in Optics, E. Wolf, ed. (North-Holland, Amsterdam, 1983), Vol. 20, Pt. 3, pp. 155–261.
  17. M. Kozierowski, “Polarization properties of hyper-Rayleigh and hyper-Raman scatterings,” in Modern Nonlinear Optics, M. Evans and S. Kielich, eds., Advances in Chemical Physics (Wiley, New York, 1993), Vol. 85, Pt. 1, pp. 127–157.
  18. V. N. Denisov, B. N. Mavrin, V. B. Podobedov, and K. E. Sterin, “Longitudinal-transverse splitting of dipole modes in hyper-Raman scattering spectra of liquid CCl4,” Opt. Commun. 44, 39–42 (1982). [CrossRef]
  19. V. N. Denisov, B. N. Mavrin, and V. B. Podobedov, “Hyper-Raman scattering by vibrational excitations in crystals, glasses and liquids,” Phys. Rep. 151, 1–92 (1987). [CrossRef]
  20. S. Kielich, M. Kozierowski, Z. Ozgo, and R. Zawodny, “Second-harmonic electric quadrupolar elastic scattering by atoms and centro-symmetric molecules,” Acta Phys. Pol. A 45, 9–19 (1974).
  21. A. D. Buckingham, “Permanent and induced molecular moments and long-range intermolecular forces,” Adv. Chem. Phys. 12, 107–142 (1967).
  22. G. Maroulis and A. J. Thakkar, “Polarizabilities and hyper-polarizabilities of carbon dioxide,” J. Chem. Phys. 93, 4164–4170 (1990). [CrossRef]
  23. D. M. Bishop and S. M. Cybulski, “Calculation of electromagnetic properties of the noble gases,” Chem. Phys. Lett. 211, 255–258 (1993). [CrossRef]
  24. S. Kielich, “Second-harmonic light scattering by dense isotropic media,” Acta Phys. Pol. A 33, 89–104 (1968).
  25. S. Kielich, “Double photon scattering by interacting qua-drupolar and octupolar molecules,” Phys. Lett. 27, 307–308 (1968). [CrossRef]
  26. S. Kielich, J. R. Lalanne, and F. B. Martin, “Second harmonic light scattering induced in liquids by quadrupolar molecules,” Acta Phys. Pol. A 41, 479–483 (1972).
  27. P. Kaatz and D. P. Shelton, “Collision induced hyper-Rayleigh light scattering in CCl4,” Mol. Phys. 88, 683–691 (1996). [CrossRef]

Cited By

Alert me when this paper is cited

OSA is able to provide readers links to articles that cite this paper by participating in CrossRef's Cited-By Linking service. CrossRef includes content from more than 3000 publishers and societies. In addition to listing OSA journal articles that cite this paper, citing articles from other participating publishers will also be listed.

Figures

Fig. 1
 

« Previous Article  |  Next Article »

OSA is a member of CrossRef.

CrossCheck Deposited