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Journal of the Optical Society of America B

Journal of the Optical Society of America B

| OPTICAL PHYSICS

  • Vol. 17, Iss. 7 — Jul. 1, 2000
  • pp: 1216–1222

Model-independent maximum-entropy method for the analysis of sum-frequency vibrational spectroscopy

Pao-Keng Yang and Jung Y. Huang  »View Author Affiliations


JOSA B, Vol. 17, Issue 7, pp. 1216-1222 (2000)
http://dx.doi.org/10.1364/JOSAB.17.001216


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Abstract

We have developed and applied a maximum-entropy phase-retrieval procedure to analyze sum-frequency vibrational spectra from a CCl4/octadecyl tricholosilane/silica interface and a hydrogen-terminated diamond C(111) surface. Some a priori knowledge of a nonlinear optical spectrum was employed for determining the phase of nonlinear optical susceptibility, and therefore the requirement for experimental phase measurement can be avoided. The results agree well with those from the Lorentzian line-shape model and justify the applicability of the a priori constraints employed in our phase-retrieval procedure.

© 2000 Optical Society of America

OCIS Codes
(190.1900) Nonlinear optics : Diagnostic applications of nonlinear optics
(190.4350) Nonlinear optics : Nonlinear optics at surfaces
(300.6490) Spectroscopy : Spectroscopy, surface

Citation
Pao-Keng Yang and Jung Y. Huang, "Model-independent maximum-entropy method for the analysis of sum-frequency vibrational spectroscopy," J. Opt. Soc. Am. B 17, 1216-1222 (2000)
http://www.opticsinfobase.org/josab/abstract.cfm?URI=josab-17-7-1216

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