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Journal of the Optical Society of America B

Journal of the Optical Society of America B

| OPTICAL PHYSICS

  • Vol. 2, Iss. 4 — Apr. 1, 1985
  • pp: 640–648

Time-domain coherent active Raman spectroscopy of a free-nitrogen jet

S. A. Akhmanov, N. I. Koroteev, S. A. Magnitskii, V. B. Morozov, A. P. Tarasevich, and V. G. Tunkin  »View Author Affiliations


JOSA B, Vol. 2, Issue 4, pp. 640-648 (1985)
http://dx.doi.org/10.1364/JOSAB.2.000640


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Abstract

A review of our results in time-domain coherent anti-Stokes Raman spectroscopy (CARS) of N2 molecules cooled in a supersonic jet is given. A full quantitative interpretation of the detected quantum beats, which makes it possible to determine the Trot of N2, is proposed. A noticeable increase of the dephasing cross section with the lowering of temperature is detected. The sensitivity of the CARS spectrometer was radically improved by the development of the injection-locked optical parametric oscillator, which made it possible to register the cooling of N2 to temperatures as low as 8 K.

© 1985 Optical Society of America

History
Original Manuscript: October 26, 1984
Manuscript Accepted: November 13, 1984
Published: April 1, 1985

Citation
S. A. Akhmanov, N. I. Koroteev, S. A. Magnitskii, V. B. Morozov, A. P. Tarasevich, and V. G. Tunkin, "Time-domain coherent active Raman spectroscopy of a free-nitrogen jet," J. Opt. Soc. Am. B 2, 640-648 (1985)
http://www.opticsinfobase.org/josab/abstract.cfm?URI=josab-2-4-640

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