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Journal of the Optical Society of America B

Journal of the Optical Society of America B


  • Vol. 20, Iss. 3 — Mar. 1, 2003
  • pp: 591–596

Quantum theory of single subfemtosecond extreme-ultraviolet pulse measurements

Markus Kitzler, Christian Fabian, Nenad Milosevic, Armin Scrinzi, and Thomas Brabec  »View Author Affiliations

JOSA B, Vol. 20, Issue 3, pp. 591-596 (2003)

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Recently the initial measurements of single attosecond pulses with laser-dressed single-photon XUV ionization of gas atoms were reported. Determination of the extreme-ultraviolet (XUV) pulse duration from the electron spectrum is based on a classical theory. Although classical models are known to give a qualitatively correct description of strong laser–atom interaction, the validity range for accurate determination of subfemtosecond pulses must be scrutinized by quantum mechanical analysis. We establish a theoretical framework for the accurate temporal characterization of attosecond XUV pulses by using a Fourier–Bessel expansion of the XUV electron spectrum under the strong field approximation and a semiclassical derivation, setting earlier results on a rigorous theoretical footing. Our analysis reveals an improved scheme that is by more than an order of magnitude more efficient than the one used so far and allows for direct experimental discrimination between single and multiple attosecond pulses.

© 2003 Optical Society of America

OCIS Codes
(260.7200) Physical optics : Ultraviolet, extreme
(320.5550) Ultrafast optics : Pulses
(320.7100) Ultrafast optics : Ultrafast measurements

Markus Kitzler, Christian Fabian, Nenad Milosevic, Armin Scrinzi, and Thomas Brabec, "Quantum theory of single subfemtosecond extreme-ultraviolet pulse measurements," J. Opt. Soc. Am. B 20, 591-596 (2003)

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  1. J. M. Schins, P. Breger, and P. Agostini, “Observation of laser-assisted auger decay in argon,” Phys. Rev. Lett. 73, 2180–2183 (1994).
  2. J. M. Schins, P. Breger, P. Agostini, R. C. Constantinescu, H. G. Muller, A. Bouhal, G. Grillon, A. Antonetti, and A. Mysyrowicz, “Cross-correlation measurements of femtosecond extreme-ultraviolet high-order harmonics,” J. Opt. Soc. Am. B 13, 197–200 (1996).
  3. T. E. Glover, R. W. Schoenlein, A. H. Chin, and C. V. Shank, “Observation of laser assisted photoelectric effect and femtosecond high order harmonic radiation,” Phys. Rev. Lett. 76, 2468–2471 (1996).
  4. A. Bouhal, R. Evans, G. Grillon, A. Mysyrowicz, P. Breger, P. Agostini, R. C. Constantinescu, H. G. Muller, and D. von der Linde, “Cross-correlation measurement of femtosecond noncollinear high-order harmonics,” J. Opt. Soc. Am. B 14, 950–956 (1997).
  5. E. Constant, V. D. Taranukhin, A. Stolow, and P. B. Corkum, “Methods for the measurement of the duration of high-harmonic pulses,” Phys. Rev. A 56, 3870–3878 (1997).
  6. A. Scrinzi, M. Geissler, and T. Brabec, “Attosecond cross correlation technique,” Phys. Rev. Lett. 86, 412–415 (2001).
  7. M. Drescher, M. Hentschel, R. Kienberger, G. Tempea, C. Spielmann, G. A. Reider, P. B. Corkum, and F. Krausz, “X-ray pulses approaching the attosecond frontier,” Science 291, 1923–1927 (2001).
  8. P. M. Paul, E. S. Toma, P. Breger, G. Mullot, F. Augé, Ph. Balcou, H. G. Muller, and P. Agostini, “Observation of a train of attosecond pulses from high harmonic generation,” Science 292, 1689–1692 (2001).
  9. E. S. Toma, H. G. Muller, P. M. Paul, P. Breger, M. Cheret, P. Agostini, C. Le Blanc, G. Mullot, and G. Cheriaux, “Ponderomotive streaking of the ionization potential as a method for measuring pulse durations in the XUV domain with fs resolution,” Phys. Rev. A 62, 061801 (R) (2000).
  10. M. Hentschel, R. Kienberger, Ch. Spielmann, G. A. Reider, N. Milosevic, T. Brabec, P. Corkum, U. Heinzmann, M. Drescher, and F. Krausz, “Attosecond metrology,” Nature 414, 509–513 (2001).
  11. V. Véniard, R. Taïeb, and A. Maquet, “Phase dependence of (N+1)-color (N>1) ir–uv photoionization of atoms with higher harmonics,” Phys. Rev. A 54, 721–728 (1996).
  12. J. Itatani, F. Quéré, G. L. Yudin, M. Yu. Ivanov, F. Krausz, and P. B. Corkum, “Attosecond streak camera,” Phys. Rev. Lett. 88, 173903 (2002).
  13. M. Kitzler, N. Milosevic, A. Scrinzi, F. Krausz, and T. Brabec, “Quantum theory of attosecond XUV pulse measurement by laser dressed photoionization,” Phys. Rev. Lett. 88, 173904 (2002).
  14. L. V. Keldysh, “Ionization in the field of a strong electromagnetic wave,” Sov. Phys. JETP 20, 1307–1314 (1965).
  15. T. Brabec and F. Krausz, “Intense few-cycle laser fields: frontiers of nonlinear optics,” Rev. Mod. Phys. 72, 545–591 (2000).
  16. U. Becker and D. A. Shirley, VUV and Soft X-Ray Photoionization (Plenum, New York, 1996).
  17. M. Abramowitz and I. A. Stegun, Handbook of Mathematical Functions (Dover, New York, 1973).
  18. C. M. Bender and S. A. Orszag, Advanced Mathematical Methods for Scientists and Engineers (McGraw Hill, New York, 1978).
  19. A. Scrinzi, T. Brabec, and M. Walser, “Momentum space description of hydrogen atom interacting with a low frequency strong laser field,” in Super-Intense Laser-Atom Physics, B. Piraux and K. Rzazewski, eds., Vol. 12 of NATO Science Series (Kluwer Academic, Dordrecht, The Netherlands, 2001), p. 313.
  20. D. B. Milosevic and F. Ehlotzky, “Coulomb and rescattering effects in above-threshold ionization,” Phys. Rev. A 58, 3124–3127 (1998).
  21. R. Kienberger, M. Hentschel, M. Uiberacker, Ch. Spielmann, M. Kitzler, A. Scrinzi, M. Wieland, Th. Westerwalbesloh, U. Kleineberg, U. Heinzmann, M. Drescher, and F. Krausz, “Steering attosecond electron wave packets with light,” Science 297, 1144–1148 (2002).

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