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Journal of the Optical Society of America B

Journal of the Optical Society of America B

| OPTICAL PHYSICS

  • Editor: G. I. Stegeman
  • Vol. 22, Iss. 11 — Nov. 1, 2005
  • pp: 2402–2408

Third-harmonic Rayleigh scattering: theory and experiment

Vladislav I. Shcheslavskiy, Solomon M. Saltiel, Alexey Faustov, Georgi I. Petrov, and Vladislav V. Yakovlev  »View Author Affiliations


JOSA B, Vol. 22, Issue 11, pp. 2402-2408 (2005)
http://dx.doi.org/10.1364/JOSAB.22.002402


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Abstract

We present an analytical model for describing optical third-harmonic generation from a sphere that is small compared with the wavelength of light. Analysis of the problem shows that the power of the third harmonic from a sphere that is small compared with the waist size and the confocal parameter of the beam is proportional to the fourth power of a sphere’s size. Experiments with different spheres both in index-matching and non-index-matching liquids are performed and confirm theoretical predictions.

© 2005 Optical Society of America

OCIS Codes
(140.7090) Lasers and laser optics : Ultrafast lasers
(190.3970) Nonlinear optics : Microparticle nonlinear optics
(190.4160) Nonlinear optics : Multiharmonic generation
(190.7110) Nonlinear optics : Ultrafast nonlinear optics
(290.5850) Scattering : Scattering, particles

ToC Category:
Scattering

Citation
Vladislav I. Shcheslavskiy, Solomon M. Saltiel, Alexey Faustov, Georgi I. Petrov, and Vladislav V. Yakovlev, "Third-harmonic Rayleigh scattering: theory and experiment," J. Opt. Soc. Am. B 22, 2402-2408 (2005)
http://www.opticsinfobase.org/josab/abstract.cfm?URI=josab-22-11-2402


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References

  1. J. W. Strut, “On the light from the sky, its polarization and color,” Philos. Mag.  41, 107–120 (1871).
  2. C. F. Bohren and D. Huffman, Absorption and Scattering of Light by Small Particles (Wiley, 1998). [CrossRef]
  3. P. W. Barber and R. K. Chang, Optical Effects Associated with Small Particles (World Scientific, 1988).
  4. X. M. Hua and J. I. Gersten, “Theory of second harmonic generation by small metal spheres,” Phys. Rev. B  33, 3756–3764 (1986). [CrossRef]
  5. H. Wang, E. Yang, E. Borguet, and K. Eisenthal, “Second harmonic generation from the surface of centrosymmetric particles in bulk solution,” Chem. Phys. Lett.  259, 15–20 (1996). [CrossRef]
  6. J. I. Dadap, J. Shan, K. B. Eisenthal, and T. F. Heinz, “Second-harmonic Rayleigh scattering from a centrosymmetric material,” Phys. Rev. Lett.  83, 4045–4048 (1999). [CrossRef]
  7. J. P. Dewitz, W. Hubner, and K. H. Bennemann, “Theory of nonlinear Mie-scattering from spherical metal clusters,” Z. Phys. D  37, 75–84 (1996). [CrossRef]
  8. J. Kasparian, B. Kramer, J. Dewitz, S. Vajda, P. Rairoux, B. Vezin, V. Boutou, T. Leisner, W. Hubner, J. Wolf, L. Woste, and K. Bennemann, “Angular dependences of third harmonic generation from microdroplets,” Phys. Rev. Lett.  78, 2952–2955 (1997). [CrossRef]
  9. D. Caroll and X. H. Zheng, “Spatial and angular distributions of third harmonic generation from metal surfaces,” Eur. Phys. J. D  5, 135–144 (1999). [CrossRef]
  10. C. Favre, V. Boutou, S. Hill, W. Zimmer, M. Krenz, H. Lambrecht, J. Yu, R. Chang, L. Woeste, and J. Wolf, “White-light nanosource with directional emission,” Phys. Rev. Lett.  89, 035002 (2002). [CrossRef] [PubMed]
  11. Z. Wang, B. Luk’yanchuk, M. Hong, Y. Lin, and T. Chong, “Energy flow around a small particle investigated by classical Mie theory,” Phys. Rev. B  70, 035418 (2004). [CrossRef]
  12. V. Shcheslavskiy, G. Petrov, S. Saltiel, and V. Yakovlev, “Quantitative characterization of aqueous solutions probed by the third-harmonic generation microscopy,” J. Struct. Biol.  147, 42–49 (2004). [CrossRef] [PubMed]
  13. M. Lippitz, M. A. van Dijk, and M. Orrit, “Third-harmonic generation from single gold nanoparticles,” Nano Lett.  5, 799–802 (2005). [CrossRef] [PubMed]
  14. L. Malmqvist and H. Hertz, “Second harmonic generation in optically trapped nonlinear particles with pulsed lasers,” Appl. Opt.  34, 3392–3397 (1995). [CrossRef] [PubMed]
  15. V. L. Brudny, B. S. Mendoza, and W. L. Mochan, “Second-harmonic generation from spherical particles,” Phys. Rev. B  62, 11152–11162 (2000). [CrossRef]
  16. J. I. Dadap, J. Shan, and T. F. Heinz, “Theory of optical second-harmonic generation from a sphere of centrosymmetric material: small-particle limit,” J. Opt. Soc. Am. B  21, 1328–1347 (2004). [CrossRef]
  17. V. I. Shcheslavskiy, G. I. Petrov, V. V. Yakovlev, S. M. Saltiel, B. S. Luk’yanchuk, Z. S. Nickolov, and J. D. Miller, “Third-harmonic generation from Rayleigh particles,” Phys. Rev. Lett., submitted for publication.
  18. J. F. Reintjes, Nonlinear Optical Parametric Processes in Liquids and Gases (Academic, 1984).
  19. S. M. Saltiel, K. Koynov, B. Agate, and W. Sibbett, “Second-harmonic generation with focused beams under conditions of large group-velocity mismatch,” J. Opt. Soc. Am. B  21, 591–598 (2004). [CrossRef]
  20. S. V. Fomichev, S. V. Popruzhenko, D. F. Zaretsky, and W. Becker, “Laser-induced nonlinear excitation of collective electron motion in a cluster,” J. Phys. B  36, 3817–3834 (2003). [CrossRef]
  21. V. Shcheslavskiy, V. Yakovlev, and A. Ivanov, “High-energy self-starting Cr4+:Mg2SiO4 oscillator operating at low repetition rate,” Opt. Lett.  26, 1999–2001 (2001). [CrossRef]
  22. V. Shcheslavskiy, G. Petrov, and V. V. Yakovlev, “Nonlinear susceptibility measurements of solutions using third-harmonic generation on the interface,” Appl. Phys. Lett.  82, 3982–3984 (2003). [CrossRef]
  23. D. Stroud and V. Wood, “Decoupling approximation for the nonlinear-optical response of composite media,” J. Opt. Soc. Am. B  6, 778–786 (1989). [CrossRef]
  24. G. I. Petrov, V. I. Shcheslavskiy, V. V. Yakovlev, I. Ozerov, E. Chelnokov, and W. Marine, “Efficient third-harmonic generation in a thin nanocrystalline film of ZnO,” Appl. Phys. Lett.  83, 3993–3995 (2003). [CrossRef]
  25. L. Malmqvist and H. M. Hertz, “Two-color trapped particle optical microscopy,” Opt. Lett.  19, 853–855 (1994). [CrossRef] [PubMed]

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