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Pump-power dependences of thermal-grating and electronic components of a polarization spectroscopy signal from dye solutions

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Abstract

Experimental evidence for different pump-power dependences of the thermal grating and the electronic contributions to a polarization spectroscopy signal is presented. This behavior, in the case of a thermal-grating signal, is interpreted as a propagation effect of the light waves along a longitudinal phase grating. In the case of the electronic signal, however, it is due to the local nonlinear interaction between the field and matter. The different pump-power dependences of the thermal and the electronic signals are used for their identification.

© 1986 Optical Society of America

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