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Journal of the Optical Society of America B

Journal of the Optical Society of America B

| OPTICAL PHYSICS

  • Editor: Grover Swartzlander
  • Vol. 30, Iss. 6 — Jun. 1, 2013
  • pp: 1486–1495

Differential cavity ring-down spectroscopy

Jérémie Courtois, Katarzyna Bielska, and Joseph T. Hodges  »View Author Affiliations


JOSA B, Vol. 30, Issue 6, pp. 1486-1495 (2013)
http://dx.doi.org/10.1364/JOSAB.30.001486


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Abstract

High-precision cavity-enhanced spectroscopic measurements are commonly compromised by interferences caused by external etalons. Here, we present the differential cavity ring-down spectroscopy (D-CRDS) technique for reducing these perturbations. We discuss how etalons are caused by coupled-cavity interactions between the primary ring-down cavity and other optical elements of the experiment, and we model and experimentally verify how drift in cavity base loss correlates with barometric pressure and laboratory temperature. D-CRDS measurements of near-infrared CO2 spectra that are insensitive to etalon-induced distortions are then presented. Based on an average of 100 spectra, these results yield a signal-to-noise ratio of 170,0001 and a minimum detectable absorption coefficient of 4×1012cm1.

© 2013 Optical Society of America

OCIS Codes
(120.6200) Instrumentation, measurement, and metrology : Spectrometers and spectroscopic instrumentation
(300.6360) Spectroscopy : Spectroscopy, laser
(300.6390) Spectroscopy : Spectroscopy, molecular

ToC Category:
Spectroscopy

History
Original Manuscript: December 19, 2012
Revised Manuscript: February 19, 2013
Manuscript Accepted: March 7, 2013
Published: May 9, 2013

Citation
Jérémie Courtois, Katarzyna Bielska, and Joseph T. Hodges, "Differential cavity ring-down spectroscopy," J. Opt. Soc. Am. B 30, 1486-1495 (2013)
http://www.opticsinfobase.org/josab/abstract.cfm?URI=josab-30-6-1486


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