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Journal of the Optical Society of America B

Journal of the Optical Society of America B

| OPTICAL PHYSICS

  • Vol. 4, Iss. 6 — Jun. 1, 1987
  • pp: 1035–1039

Resonant third-order hyperpolarizabilities of large organic molecules

C. Maloney and W. Blau  »View Author Affiliations


JOSA B, Vol. 4, Issue 6, pp. 1035-1039 (1987)
http://dx.doi.org/10.1364/JOSAB.4.001035


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Abstract

Resonant degenerate four-wave mixing in a number of infrared-absorbing dyeswas studied with 160-psec pulses at 1.064 µm. Hyperpolarizabilities in the range of 10-44 to 10-42 V-2 m5 were observed. A theoretical model based on a two-band system is developed that explains the results and permits the prediction of hyperpolarizabilities from the linear spectroscopic properties.

© 1987 Optical Society of America

Citation
C. Maloney and W. Blau, "Resonant third-order hyperpolarizabilities of large organic molecules," J. Opt. Soc. Am. B 4, 1035-1039 (1987)
http://www.opticsinfobase.org/josab/abstract.cfm?URI=josab-4-6-1035

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