Third-order nonlinear optical properties exhibited by a bilayer configuration of silver nanoparticles integrated to silicon nanocrystals embedded in ion-implanted silica

Alejandra López-Suárez; Carlos Torres-Torres; Bonifacio Can-Uc; Raúl Rangel-Rojo; Carlos E. Valencia; Alicia Oliver

doi:10.1364/JOSAB.32.000805

Journal of the Optical Society of America B
Vol. 32,
Issue 5,
pp. 805-811
(2015)
•https://doi.org/10.1364/JOSAB.32.000805

Third-order nonlinear optical properties exhibited by a bilayer configuration of silver nanoparticles integrated to silicon nanocrystals embedded in ion-implanted silica

Alejandra López-Suárez, Carlos Torres-Torres, Bonifacio Can-Uc, Raúl Rangel-Rojo, Carlos E. Valencia, and Alicia Oliver

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Alejandra López-Suárez, Carlos Torres-Torres, Bonifacio Can-Uc, Raúl Rangel-Rojo, Carlos E. Valencia, and Alicia Oliver, "Third-order nonlinear optical properties exhibited by a bilayer configuration of silver nanoparticles integrated to silicon nanocrystals embedded in ion-implanted silica," J. Opt. Soc. Am. B 32, 805-811 (2015)

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Abstract

We present the optical Kerr effect, and nonlinear optical absorption studies of two closely spaced distributions of silver nanoparticles embedded in silica containing ion-implanted silicon nanocrystals. The z-scan technique was used to explore the third-order optical nonlinear response at 830 nm with 80 fs pulses. Two-wave mixing experiments were comparatively examined by a vectorial method at 532 nm wavelength using nanosecond pulses. The femtosecond results reveal that both saturated and two-photon absorption seem to contribute to the nonlinear absorption observed. From nanosecond observations, we identify that a remarkable enhancement in the third-order optical nonlinearity is achieved by the double-implantation process.

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	Silver Implantation Fluence ( $Ag / {cm}^{2}$ )
Sample	Energy Implantation 1 MeV	Energy Implantation 3 MeV
Ag ions 1 MeV+ Ag ions 3 MeV+ Si 5 MeV	$3.92 \times 10^{16}$	$2.6 \times 10^{16}$
Ag ions 1 MeV+ Si 5 MeV	$6.32 \times 10^{16}$
Ag ions 3 MeV+ Si 5 MeV		$5.75 \times 10^{16}$

	Nonlinear Optical Response at $λ = 825 nm$ , $t = 80 fs$			Nonlinear Optical Response at $λ = 532 nm$ , $t = 1 ns$
Sample	$n_{2}$ [ $m^{2} / W$ ]	$β$ [m/W]	$\| χ^{(3)} \|$ [esu]	$\| χ^{(3)} \|$ [esu]
Bi-Ag	$1.88 \times 10^{- 14}$	$- 2.576 \times 10^{- 8}$	$1.9310 \times 10^{- 9}$	$9.2 \times 10^{- 8}$
1M-Ag	$3.35 \times 10^{- 14}$	0	$2.5619 \times 10^{- 9}$	$1.4 \times 10^{- 8}$
3M-Ag	$2.31 \times 10^{- 14}$	$9.39 \times 10^{- 8}$	$5.0258 \times 10^{- 9}$	$3.1 \times 10^{- 8}$

	Silver Implantation Fluence ( $Ag / {cm}^{2}$ )
Sample	Energy Implantation 1 MeV	Energy Implantation 3 MeV
Ag ions 1 MeV+ Ag ions 3 MeV+ Si 5 MeV	$3.92 \times 10^{16}$	$2.6 \times 10^{16}$
Ag ions 1 MeV+ Si 5 MeV	$6.32 \times 10^{16}$
Ag ions 3 MeV+ Si 5 MeV		$5.75 \times 10^{16}$

	Nonlinear Optical Response at $λ = 825 nm$ , $t = 80 fs$			Nonlinear Optical Response at $λ = 532 nm$ , $t = 1 ns$
Sample	$n_{2}$ [ $m^{2} / W$ ]	$β$ [m/W]	$\| χ^{(3)} \|$ [esu]	$\| χ^{(3)} \|$ [esu]
Bi-Ag	$1.88 \times 10^{- 14}$	$- 2.576 \times 10^{- 8}$	$1.9310 \times 10^{- 9}$	$9.2 \times 10^{- 8}$
1M-Ag	$3.35 \times 10^{- 14}$	0	$2.5619 \times 10^{- 9}$	$1.4 \times 10^{- 8}$
3M-Ag	$2.31 \times 10^{- 14}$	$9.39 \times 10^{- 8}$	$5.0258 \times 10^{- 9}$	$3.1 \times 10^{- 8}$

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