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On the question of pulsed laser cooling. Collective luminescence and light quenching in high-concentration solutions of rhodamine 101

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Abstract

The transmittance and luminescence of concentrated solutions of rhodamine 101 excited by laser pulses in the Stokes and anti-Stoke regions of the spectrum have been experimentally investigated. It is shown that a substantial role in forming the luminescence is played at large pump energies by collective photoinduced luminescence, which competes with induced emission. Estimates are made of the heating and cooling of solutions. © 2005 Optical Society of America

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