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Optics Express

Optics Express

  • Editor: C. Martijn de Sterke
  • Vol. 15, Iss. 22 — Oct. 29, 2007
  • pp: 14289–14298

Localized plasmon-engineered spontaneous emission of CdSe/ZnS nanocrystals closely-packed in the proximity of Ag nanoisland films for controlling emission linewidth, peak, and intensity

Ibrahim Murat Soganci, Sedat Nizamoglu, Evren Mutlugun, Onur Akin, and Hilmi Volkan Demir  »View Author Affiliations


Optics Express, Vol. 15, Issue 22, pp. 14289-14298 (2007)
http://dx.doi.org/10.1364/OE.15.014289


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Abstract

Using metallic nanoislands, we demonstrate the localized plasmonic control and modification of the spontaneous emission from closely-packed nanocrystal emitters, leading to significant changes in their collective emission characteristics tuned spectrally and spatially by plasmon coupling. Using randomly-distributed silver nanoislands, we show that the emission linewidth of proximal CdSe/ZnS core-shell quantum dots is reduced by 22% and their peak emission wavelength is shifted by 14nm, while their ensemble photoluminescence is enhanced via radiative energy transfer by 21.6 and 15.1 times compared to the control groups of CdSe/ZnS nanocrystals with identical nano-silver but no dielectric spacer and the same nanocrystals alone, respectively.

© 2007 Optical Society of America

OCIS Codes
(160.2540) Materials : Fluorescent and luminescent materials
(240.6680) Optics at surfaces : Surface plasmons
(250.5230) Optoelectronics : Photoluminescence
(260.3910) Physical optics : Metal optics
(310.1860) Thin films : Deposition and fabrication
(310.6860) Thin films : Thin films, optical properties

ToC Category:
Optics at Surfaces

History
Original Manuscript: August 8, 2007
Revised Manuscript: October 8, 2007
Manuscript Accepted: October 9, 2007
Published: October 15, 2007

Virtual Issues
Vol. 2, Iss. 11 Virtual Journal for Biomedical Optics

Citation
Ibrahim M. Soganci, Sedat Nizamoglu, Evren Mutlugun, Onur Akin, and Hilmi V. Demir, "Localized plasmon-engineered spontaneous emission of CdSe/ZnS nanocrystals closely-packed in the proximity of Ag nanoisland films for controlling emission linewidth, peak, and intensity," Opt. Express 15, 14289-14298 (2007)
http://www.opticsinfobase.org/oe/abstract.cfm?URI=oe-15-22-14289


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