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Wavelength effect on atomic and molecular high harmonic generation driven by a tunable infrared parametric source
Pengfei Wei, Chunmei Zhang, Candong Liu, Yansui Huang, Yuxin Leng, Peng Liu, Yinghui Zheng, Zhinan Zeng, Ruxin Li, and Zhizhan Xu »View Author Affiliations
State Key Laboratory of High Field Laser Physics, Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Shanghai 201800, China
*Corresponding author: lengyuxin@siom.ac.cn
Optics Express, Vol. 17, Issue 17, pp. 15061-15067 (2009)
http://dx.doi.org/10.1364/OE.17.015061
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Abstract
We experimentally investigate the wavelength effect on high-order harmonic generation (HHG) in CH4 molecules and Xe atoms driven by a tunable infrared parametric source, and observe that the molecular HHG around the vibrational resonance is more sensitive to the driver wavelength than HHG from an atomic gas with comparable ionization potential. The results can be attributed to the light nuclear motion induced by the driving laser field, and it becomes possible to control the proton vibration in the molecular HHG by tuning the infrared wavelength of the driving laser.
© 2009 OSA
OCIS Codes
(190.2620) Nonlinear optics : Harmonic generation and mixing
(020.2649) Atomic and molecular physics : Strong field laser physics
ToC Category:
Atomic and Molecular Physics
History
Original Manuscript: June 19, 2009
Revised Manuscript: July 30, 2009
Manuscript Accepted: August 4, 2009
Published: August 10, 2009
Citation
Pengfei Wei, Chunmei Zhang, Candong Liu, Yansui Huang, Yuxin Leng, Peng Liu, Yinghui Zheng, Zhinan Zeng, Ruxin Li, and Zhizhan Xu, "Wavelength effect on atomic and molecular high harmonic generation driven by a tunable infrared parametric source," Opt. Express 17, 15061-15067 (2009)
http://www.opticsinfobase.org/oe/abstract.cfm?URI=oe-17-17-15061
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References
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- C. Vozzi, F. Calegari, E. Benedetti, J.-P. Caumes, G. Sansone, S. Stagira, M. Nisoli, C. Altucci, and R. Velotta, “Controlling two-center interference in molecular high harmonic generation,” Phys. Rev. Lett. 95(15), 153902 (2005). [CrossRef] [PubMed]
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- A. D. Bandrauk, S. Chelkowski, S. Kawai, and H. Lu, “Effect of nuclear motion on molecular high-order harmonics and on generation of attosecond pulses in intense laser pulses,” Phys. Rev. Lett. 101(15), 153901 (2008). [CrossRef] [PubMed]
- C. Vozzi, F. Calegari, E. Benedetti, S. Gasilov, G. Sansone, G. Cerullo, M. Nisoli, S. De Silvestri, and S. Stagira, “Millijoule-level phase-stabilized few-optical-cycle infrared parametric source,” Opt. Lett. 32(20), 2957–2959 (2007). [CrossRef] [PubMed]
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- C. Vozzi, F. Calegari, E. Benedetti, J.-P. Caumes, G. Sansone, S. Stagira, M. Nisoli, C. Altucci, and R. Velotta, “Controlling two-center interference in molecular high harmonic generation,” Phys. Rev. Lett. 95(15), 153902 (2005). [CrossRef] [PubMed]
- P. Colosimo, G. Doumy, C. Blaga, J. Wheeler, C. Hauri, F. Catoire, J. Tate, R. Chirla, A. March, G. Paulus, H. Muller, P. Agostini, and L. Dimauro, “Scaling strong-field interactions towards the classical limit,” Nat. Phys. 4(5), 386–389 (2008). [CrossRef]
- M. Hentschel, R. Kienberger, C. Spielmann, G. A. Reider, N. Milosevic, T. Brabec, P. Corkum, U. Heinzmann, M. Drescher, and F. Krausz, “Attosecond metrology,” Nature 414(6863), 509–513 (2001). [CrossRef] [PubMed]
- C. Vozzi, F. Calegari, E. Benedetti, S. Gasilov, G. Sansone, G. Cerullo, M. Nisoli, S. De Silvestri, and S. Stagira, “Millijoule-level phase-stabilized few-optical-cycle infrared parametric source,” Opt. Lett. 32(20), 2957–2959 (2007). [CrossRef] [PubMed]
- C. Vozzi, G. Cirmi, C. Manzoni, E. Benedetti, F. Calegari, G. Sansone, S. Stagira, O. Svelto, S. De Silvestri, M. Nisoli, and G. Cerullo, “High-energy, few-optical-cycle pulses at 1.5 µm with passive carrier-envelope phase stabilization,” Opt. Express 14(21), 10109–10116 (2006). [CrossRef] [PubMed]
- G. Sansone, E. Benedetti, F. Calegari, C. Vozzi, L. Avaldi, R. Flammini, L. Poletto, P. Villoresi, C. Altucci, R. Velotta, S. Stagira, S. De Silvestri, and M. Nisoli, “Isolated single-cycle attosecond pulses,” Science 314(5798), 443–446 (2006). [CrossRef] [PubMed]
- C. Vozzi, F. Calegari, E. Benedetti, J.-P. Caumes, G. Sansone, S. Stagira, M. Nisoli, C. Altucci, and R. Velotta, “Controlling two-center interference in molecular high harmonic generation,” Phys. Rev. Lett. 95(15), 153902 (2005). [CrossRef] [PubMed]
- R. de Nalda, E. Heesel, M. Lein, N. Hay, R. Velotta, E. Springate, M. Castillejo, and J. P. Marangos, “Role of orbital symmetry in high-order harmonic generation from aligned molecules,” Phys. Rev. A 69(3), 031804 (2004). [CrossRef]
- P. Colosimo, G. Doumy, C. Blaga, J. Wheeler, C. Hauri, F. Catoire, J. Tate, R. Chirla, A. March, G. Paulus, H. Muller, P. Agostini, and L. Dimauro, “Scaling strong-field interactions towards the classical limit,” Nat. Phys. 4(5), 386–389 (2008). [CrossRef]
- C. Vozzi, F. Calegari, E. Benedetti, J.-P. Caumes, G. Sansone, S. Stagira, M. Nisoli, C. Altucci, and R. Velotta, “Controlling two-center interference in molecular high harmonic generation,” Phys. Rev. Lett. 95(15), 153902 (2005). [CrossRef] [PubMed]
- C. Vozzi, F. Calegari, E. Benedetti, S. Gasilov, G. Sansone, G. Cerullo, M. Nisoli, S. De Silvestri, and S. Stagira, “Millijoule-level phase-stabilized few-optical-cycle infrared parametric source,” Opt. Lett. 32(20), 2957–2959 (2007). [CrossRef] [PubMed]
- C. Vozzi, G. Cirmi, C. Manzoni, E. Benedetti, F. Calegari, G. Sansone, S. Stagira, O. Svelto, S. De Silvestri, M. Nisoli, and G. Cerullo, “High-energy, few-optical-cycle pulses at 1.5 µm with passive carrier-envelope phase stabilization,” Opt. Express 14(21), 10109–10116 (2006). [CrossRef] [PubMed]
- A. D. Bandrauk, S. Chelkowski, S. Kawai, and H. Lu, “Effect of nuclear motion on molecular high-order harmonics and on generation of attosecond pulses in intense laser pulses,” Phys. Rev. Lett. 101(15), 153901 (2008). [CrossRef] [PubMed]
- P. Wei, P. Liu, J. Chen, Z. Zeng, X. Guo, X. Ge, R. Li, and Z. Xu, “Laser-field-related recombination interference in high-order harmonic generation from CO2 molecules,” Phys. Rev. A 79(5), 053814 (2009). [CrossRef]
- S. Baker, J. S. Robinson, C. A. Haworth, H. Teng, R. A. Smith, C. C. Chirilã, M. Lein, J. W. G. Tisch, and J. P. Marangos, “Probing proton dynamics in molecules on an attosecond time scale,” Science 312(5772), 424–427 (2006). [CrossRef] [PubMed]
- P. Colosimo, G. Doumy, C. Blaga, J. Wheeler, C. Hauri, F. Catoire, J. Tate, R. Chirla, A. March, G. Paulus, H. Muller, P. Agostini, and L. Dimauro, “Scaling strong-field interactions towards the classical limit,” Nat. Phys. 4(5), 386–389 (2008). [CrossRef]
- N. L. Wagner, A. Wüest, I. P. Christov, T. Popmintchev, X. Zhou, M. M. Murnane, and H. C. Kapteyn, “Monitoring molecular dynamics using coherent electrons from high harmonic generation,” Proc. Natl. Acad. Sci. U.S.A. 103(36), 13279–13285 (2006). [CrossRef] [PubMed]
- P. Colosimo, G. Doumy, C. Blaga, J. Wheeler, C. Hauri, F. Catoire, J. Tate, R. Chirla, A. March, G. Paulus, H. Muller, P. Agostini, and L. Dimauro, “Scaling strong-field interactions towards the classical limit,” Nat. Phys. 4(5), 386–389 (2008). [CrossRef]
- M. Hentschel, R. Kienberger, C. Spielmann, G. A. Reider, N. Milosevic, T. Brabec, P. Corkum, U. Heinzmann, M. Drescher, and F. Krausz, “Attosecond metrology,” Nature 414(6863), 509–513 (2001). [CrossRef] [PubMed]
- J. Itatani, D. Zeidler, J. Levesque, M. Spanner, D. M. Villeneuve, and P. B. Corkum, “Controlling high harmonic generation with molecular wave packets,” Phys. Rev. Lett. 94(12), 123902 (2005). [CrossRef] [PubMed]
- J. Itatani, J. Levesque, D. Zeidler, H. Niikura, H. Pépin, J. C. Kieffer, P. B. Corkum, and D. M. Villeneuve, “Tomographic imaging of molecular orbitals,” Nature 432(7019), 867–871 (2004). [CrossRef] [PubMed]
- M. Yu. Ivanov and P. B. Corkum, “Generation of high-order harmonics from inertially confined molecular ions,” Phys. Rev. A 48(1), 580–590 (1993). [CrossRef] [PubMed]
- P. B. Corkum, “Plasma perspective on strong field multiphoton ionization,” Phys. Rev. Lett. 71(13), 1994–1997 (1993). [CrossRef] [PubMed]
- R. de Nalda, E. Heesel, M. Lein, N. Hay, R. Velotta, E. Springate, M. Castillejo, and J. P. Marangos, “Role of orbital symmetry in high-order harmonic generation from aligned molecules,” Phys. Rev. A 69(3), 031804 (2004). [CrossRef]
- C. Vozzi, F. Calegari, E. Benedetti, S. Gasilov, G. Sansone, G. Cerullo, M. Nisoli, S. De Silvestri, and S. Stagira, “Millijoule-level phase-stabilized few-optical-cycle infrared parametric source,” Opt. Lett. 32(20), 2957–2959 (2007). [CrossRef] [PubMed]
- C. Vozzi, G. Cirmi, C. Manzoni, E. Benedetti, F. Calegari, G. Sansone, S. Stagira, O. Svelto, S. De Silvestri, M. Nisoli, and G. Cerullo, “High-energy, few-optical-cycle pulses at 1.5 µm with passive carrier-envelope phase stabilization,” Opt. Express 14(21), 10109–10116 (2006). [CrossRef] [PubMed]
- G. Sansone, E. Benedetti, F. Calegari, C. Vozzi, L. Avaldi, R. Flammini, L. Poletto, P. Villoresi, C. Altucci, R. Velotta, S. Stagira, S. De Silvestri, and M. Nisoli, “Isolated single-cycle attosecond pulses,” Science 314(5798), 443–446 (2006). [CrossRef] [PubMed]
- P. Colosimo, G. Doumy, C. Blaga, J. Wheeler, C. Hauri, F. Catoire, J. Tate, R. Chirla, A. March, G. Paulus, H. Muller, P. Agostini, and L. Dimauro, “Scaling strong-field interactions towards the classical limit,” Nat. Phys. 4(5), 386–389 (2008). [CrossRef]
- J. Tate, T. Auguste, H. G. Muller, P. Salières, P. Agostini, and L. F. DiMauro, “Scaling of wave-packet dynamics in an intense midinfrared field,” Phys. Rev. Lett. 98(1), 013901 (2007). [CrossRef] [PubMed]
- P. Colosimo, G. Doumy, C. Blaga, J. Wheeler, C. Hauri, F. Catoire, J. Tate, R. Chirla, A. March, G. Paulus, H. Muller, P. Agostini, and L. Dimauro, “Scaling strong-field interactions towards the classical limit,” Nat. Phys. 4(5), 386–389 (2008). [CrossRef]
- M. Hentschel, R. Kienberger, C. Spielmann, G. A. Reider, N. Milosevic, T. Brabec, P. Corkum, U. Heinzmann, M. Drescher, and F. Krausz, “Attosecond metrology,” Nature 414(6863), 509–513 (2001). [CrossRef] [PubMed]
- M. Frolov, N. Manakov, T. Sarantseva, M. Emelin, M. Ryabikin, and A. Starace, “Analytic Description of the High-Energy Plateau in Harmonic Generation by Atoms: Can the Harmonic Power Increase with Increasing Laser Wavelengths?” Phys. Rev. Lett. 102(24), 243901 (2009). [CrossRef] [PubMed]
- G. Sansone, E. Benedetti, F. Calegari, C. Vozzi, L. Avaldi, R. Flammini, L. Poletto, P. Villoresi, C. Altucci, R. Velotta, S. Stagira, S. De Silvestri, and M. Nisoli, “Isolated single-cycle attosecond pulses,” Science 314(5798), 443–446 (2006). [CrossRef] [PubMed]
- M. Frolov, N. Manakov, T. Sarantseva, M. Emelin, M. Ryabikin, and A. Starace, “Analytic Description of the High-Energy Plateau in Harmonic Generation by Atoms: Can the Harmonic Power Increase with Increasing Laser Wavelengths?” Phys. Rev. Lett. 102(24), 243901 (2009). [CrossRef] [PubMed]
- P. Wei, P. Liu, J. Chen, Z. Zeng, X. Guo, X. Ge, R. Li, and Z. Xu, “Laser-field-related recombination interference in high-order harmonic generation from CO2 molecules,” Phys. Rev. A 79(5), 053814 (2009). [CrossRef]
- P. Liu, P. Yu, Z. Zeng, H. Xiong, X. Ge, R. Li, and Z. Xu, “Laser intensity dependence of high-order harmonic generation from aligned CO2 molecules,” Phys. Rev. A 78(1), 015802 (2008). [CrossRef]
- P. Wei, P. Liu, J. Chen, Z. Zeng, X. Guo, X. Ge, R. Li, and Z. Xu, “Laser-field-related recombination interference in high-order harmonic generation from CO2 molecules,” Phys. Rev. A 79(5), 053814 (2009). [CrossRef]
- P. Colosimo, G. Doumy, C. Blaga, J. Wheeler, C. Hauri, F. Catoire, J. Tate, R. Chirla, A. March, G. Paulus, H. Muller, P. Agostini, and L. Dimauro, “Scaling strong-field interactions towards the classical limit,” Nat. Phys. 4(5), 386–389 (2008). [CrossRef]
- S. Baker, J. S. Robinson, C. A. Haworth, H. Teng, R. A. Smith, C. C. Chirilã, M. Lein, J. W. G. Tisch, and J. P. Marangos, “Probing proton dynamics in molecules on an attosecond time scale,” Science 312(5772), 424–427 (2006). [CrossRef] [PubMed]
- R. de Nalda, E. Heesel, M. Lein, N. Hay, R. Velotta, E. Springate, M. Castillejo, and J. P. Marangos, “Role of orbital symmetry in high-order harmonic generation from aligned molecules,” Phys. Rev. A 69(3), 031804 (2004). [CrossRef]
- R. de Nalda, E. Heesel, M. Lein, N. Hay, R. Velotta, E. Springate, M. Castillejo, and J. P. Marangos, “Role of orbital symmetry in high-order harmonic generation from aligned molecules,” Phys. Rev. A 69(3), 031804 (2004). [CrossRef]
- M. Hentschel, R. Kienberger, C. Spielmann, G. A. Reider, N. Milosevic, T. Brabec, P. Corkum, U. Heinzmann, M. Drescher, and F. Krausz, “Attosecond metrology,” Nature 414(6863), 509–513 (2001). [CrossRef] [PubMed]
- M. Hentschel, R. Kienberger, C. Spielmann, G. A. Reider, N. Milosevic, T. Brabec, P. Corkum, U. Heinzmann, M. Drescher, and F. Krausz, “Attosecond metrology,” Nature 414(6863), 509–513 (2001). [CrossRef] [PubMed]
- C. Zhang, P. Wei, Y. Huang, Y. Leng, Y. Zheng, Z. Zeng, R. Li, and Z. Xu, “Tunable phase-stabilized infrared optical parametric amplifier for high order harmonic generation,” Opt. Lett. Submitted. [PubMed]
- J. Itatani, D. Zeidler, J. Levesque, M. Spanner, D. M. Villeneuve, and P. B. Corkum, “Controlling high harmonic generation with molecular wave packets,” Phys. Rev. Lett. 94(12), 123902 (2005). [CrossRef] [PubMed]
- J. Itatani, J. Levesque, D. Zeidler, H. Niikura, H. Pépin, J. C. Kieffer, P. B. Corkum, and D. M. Villeneuve, “Tomographic imaging of molecular orbitals,” Nature 432(7019), 867–871 (2004). [CrossRef] [PubMed]
- M. Yu. Ivanov and P. B. Corkum, “Generation of high-order harmonics from inertially confined molecular ions,” Phys. Rev. A 48(1), 580–590 (1993). [CrossRef] [PubMed]
- T. Kanai, S. Minemoto, and H. Sakai, “Quantum interference during high-order harmonic generation from aligned molecules,” Nature 435(7041), 470–474 (2005). [CrossRef] [PubMed]
- N. L. Wagner, A. Wüest, I. P. Christov, T. Popmintchev, X. Zhou, M. M. Murnane, and H. C. Kapteyn, “Monitoring molecular dynamics using coherent electrons from high harmonic generation,” Proc. Natl. Acad. Sci. U.S.A. 103(36), 13279–13285 (2006). [CrossRef] [PubMed]
- A. D. Bandrauk, S. Chelkowski, S. Kawai, and H. Lu, “Effect of nuclear motion on molecular high-order harmonics and on generation of attosecond pulses in intense laser pulses,” Phys. Rev. Lett. 101(15), 153901 (2008). [CrossRef] [PubMed]
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Chin. Phys. Lett.
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Nat. Phys.
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