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Optics Express

Optics Express

  • Editor: C. Martijn de Sterke
  • Vol. 18, Iss. 22 — Oct. 25, 2010
  • pp: 23302–23313

Optimized nanospherical layered alternating metal-dielectric probes for optical sensing

Anil K. Kodali, Matthew V. Schulmerich, Rohun Palekar, Xavier Llora, and Rohit Bhargava  »View Author Affiliations


Optics Express, Vol. 18, Issue 22, pp. 23302-23313 (2010)
http://dx.doi.org/10.1364/OE.18.023302


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Abstract

Multishell nanospheres have been proposed as a class of layered alternating metal-dielectric probes (LAMPs) that can greatly enhance sensitivity and multiplexing capabilities of optical molecular imaging . Here we theoretically demonstrate that the interplasmonic coupling within these spheres and hence their spectral responses can be tuned by a rational selection of layer thicknesses. As a proof-of-concept, layered Mie theory calculations of near- and far-field characteristics followed by a genetic algorithm-based selection are presented for gold-silica, silver-silica and copper-silica LAMPs. The results demonstrate that the optical tunability available allows for design of application (excitation wavelength)-specific probes of different sizes. The tunability further increases with number of layers and within a particular allowable probe size provides for structures with distinct resonances at longer wavelengths. The concept of scaling internal field resonances is also shown theoretically and the range over which the magnitudes can be tuned are presented.

© 2010 OSA

OCIS Codes
(160.4760) Materials : Optical properties
(240.6680) Optics at surfaces : Surface plasmons
(300.6550) Spectroscopy : Spectroscopy, visible
(350.4600) Other areas of optics : Optical engineering
(160.4236) Materials : Nanomaterials
(350.4238) Other areas of optics : Nanophotonics and photonic crystals
(280.4788) Remote sensing and sensors : Optical sensing and sensors
(240.6695) Optics at surfaces : Surface-enhanced Raman scattering

ToC Category:
Optics at Surfaces

History
Original Manuscript: August 13, 2010
Revised Manuscript: September 23, 2010
Manuscript Accepted: September 23, 2010
Published: October 20, 2010

Virtual Issues
Vol. 6, Iss. 1 Virtual Journal for Biomedical Optics

Citation
Anil K. Kodali, Matthew V. Schulmerich, Rohun Palekar, Xavier Llora, and Rohit Bhargava, "Optimized nanospherical layered alternating metal-dielectric probes for optical sensing," Opt. Express 18, 23302-23313 (2010)
http://www.opticsinfobase.org/oe/abstract.cfm?URI=oe-18-22-23302


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