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Optical properties of ordered vertical arrays of multi-walled carbon nanotubes from FDTD simulations
Hua Bao, Xiulin Ruan, and Timothy S. Fisher »View Author Affiliations
Hua Bao,
Xiulin Ruan,*
and Timothy S. Fisher
School of Mechanical Engineering, Birck Nanotechnology Center, and Energy Center Purdue University, West Lafayette, Indiana 47907-2088
*ruan@purdue.edu
Optics Express, Vol. 18, Issue 6, pp. 6347-6359 (2010)
http://dx.doi.org/10.1364/OE.18.006347
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Abstract
A finite-difference time-domain (FDTD) method is used to model thermal radiative properties of vertical arrays of multi-walled carbon nanotubes (MWCNT). Individual CNTs are treated as solid circular cylinders with an effective dielectric tensor. Consistent with experiments, the results confirm that CNT arrays are highly absorptive. Compared with the commonly used Maxwell-Garnett theory, the FDTD calculations generally predict larger reflectance and absorbance, and smaller transmittance, which are attributed to the diffraction and scattering within the cylinder array structure. The effects of volume fraction, tube length, tube distance, and incident angle on radiative properties are investigated systematically. Low volume fraction and long tubes are more favorable to achieve low reflectance and high absorbance. For a fixed volume fraction and finite tube length, larger periodicity results in larger reflectance and absorbance. The angular dependence studies reveal an optimum incident angle at which the reflectance can be minimized. The results also suggest that an even darker material could be achieved by using CNTs with good alignment on the top surface.
© 2010 Optical Society of America
OCIS Codes
(310.6628) Thin films : Subwavelength structures, nanostructures
ToC Category:
Thin Films
History
Original Manuscript: January 15, 2010
Revised Manuscript: February 23, 2010
Manuscript Accepted: March 3, 2010
Published: March 12, 2010
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Focus Issue: Solar Concentrators (2010) Optics Express
Citation
Hua Bao, Xiulin Ruan, and Timothy S. Fisher, "Optical properties of ordered vertical arrays of multi-walled carbon nanotubes from FDTD simulations," Opt. Express 18, 6347-6359 (2010)
http://www.opticsinfobase.org/oe/abstract.cfm?URI=oe-18-6-6347
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References
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