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Optics Express

Optics Express

  • Editor: C. Martijn de Sterke
  • Vol. 20, Iss. 19 — Sep. 10, 2012
  • pp: 20908–20919

Modeling and correction of distorted two-dimensional Fourier transform spectra from pixelated pulse shaping devices

Erik M. Grumstrup and Niels H. Damrauer  »View Author Affiliations


Optics Express, Vol. 20, Issue 19, pp. 20908-20919 (2012)
http://dx.doi.org/10.1364/OE.20.020908


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Abstract

Two-dimensional Fourier transform spectra of a three level model system are simulated using a non-perturbative density matrix formalism. The electric field distortions resultant from using pixelated pulse shaping devices to produce phase-locked pulse pairs are modeled and the effects on the recovered spectra are examined. To minimize spectral distortions, a temporal filtering scheme is employed which eliminates contributions from spurious sample polarizations.

© 2012 OSA

OCIS Codes
(020.0020) Atomic and molecular physics : Atomic and molecular physics
(070.0070) Fourier optics and signal processing : Fourier optics and signal processing
(300.0300) Spectroscopy : Spectroscopy

ToC Category:
Spectroscopy

History
Original Manuscript: June 7, 2012
Revised Manuscript: August 7, 2012
Manuscript Accepted: August 21, 2012
Published: August 28, 2012

Citation
Erik M. Grumstrup and Niels H. Damrauer, "Modeling and correction of distorted two-dimensional Fourier transform spectra from pixelated pulse shaping devices," Opt. Express 20, 20908-20919 (2012)
http://www.opticsinfobase.org/oe/abstract.cfm?URI=oe-20-19-20908


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References

  1. J. D. Hybl, A. W. Albrecht, S. M. Gallagher Faeder, and D. M. Jonas, “Two-dimensional electronic spectroscopy,” Chem. Phys. Lett.297(3-4), 307–313 (1998). [CrossRef]
  2. I. Stiopkin, T. Brixner, M. Yang, and G. R. Fleming, “Heterogeneous exciton dynamics revealed by two-dimensional optical spectroscopy,” J. Phys. Chem. B110(40), 20032–20037 (2006). [CrossRef] [PubMed]
  3. G. S. Engel, T. R. Calhoun, E. L. Read, T.-K. Ahn, T. Mančal, Y.-C. Cheng, R. E. Blankenship, and G. R. Fleming, “Evidence for wavelike energy transfer through quantum coherence in photosynthetic systems,” Nature446(7137), 782–786 (2007). [CrossRef] [PubMed]
  4. D. Zigmantas, E. L. Read, T. Mančal, T. Brixner, A. T. Gardiner, R. J. Cogdell, and G. R. Fleming, “Two-dimensional electronic spectroscopy of the B800-B820 light-harvesting complex,” Proc. Natl. Acad. Sci. U.S.A.103(34), 12672–12677 (2006). [CrossRef] [PubMed]
  5. P. Tian, D. Keusters, Y. Suzaki, and W. S. Warren, “Femtosecond phase-coherent two-dimensional spectroscopy,” Science300(5625), 1553–1555 (2003). [CrossRef] [PubMed]
  6. W. Wagner, C. Li, J. Semmlow, and W. Warren, “Rapid phase-cycled two-dimensional optical spectroscopy in fluorescence and transmission mode,” Opt. Express13(10), 3697–3706 (2005). [CrossRef] [PubMed]
  7. S. H. Shim, D. B. Strasfeld, E. C. Fulmer, and M. T. Zanni, “Femtosecond pulse shaping directly in the mid-IR using acousto-optic modulation,” Opt. Lett.31(6), 838–840 (2006). [CrossRef] [PubMed]
  8. S. H. Shim, D. B. Strasfeld, Y. L. Ling, and M. T. Zanni, “Automated 2D IR spectroscopy using a mid-IR pulse shaper and application of this technology to the human islet amyloid polypeptide,” Proc. Natl. Acad. Sci. U.S.A.104(36), 14197–14202 (2007). [CrossRef] [PubMed]
  9. E. M. Grumstrup, S.-H. Shim, M. A. Montgomery, N. H. Damrauer, and M. T. Zanni, “Facile collection of two-dimensional electronic spectra using femtosecond pulse-shaping technology,” Opt. Express15(25), 16681–16689 (2007). [CrossRef] [PubMed]
  10. J. A. Myers, K. L. M. Lewis, P. F. Tekavec, and J. P. Ogilvie, “Two-color two-dimensional Fourier transform electronic spectroscopy with a pulse-shaper,” Opt. Express16(22), 17420–17428 (2008). [CrossRef] [PubMed]
  11. P. F. Tekavec, J. A. Myers, K. L. M. Lewis, and J. P. Ogilvie, “Two-dimensional electronic spectroscopy with a continuum probe,” Opt. Lett.34(9), 1390–1392 (2009). [CrossRef] [PubMed]
  12. P. F. Tekavec, J. A. Myers, K. L. M. Lewis, F. D. Fuller, and J. P. Ogilvie, “Effects of chirp on two-dimensional Fourier transform electronic spectra,” Opt. Express18(11), 11015–11024 (2010). [CrossRef] [PubMed]
  13. M. Kullmann, S. Ruetzel, J. Buback, P. Nuernberger, and T. Brixner, “Reaction dynamics of a molecular switch unveiled by coherent two-dimensional electronic spectroscopy,” J. Am. Chem. Soc.133(33), 13074–13080 (2011). [CrossRef] [PubMed]
  14. K. L. M. Lewis and J. P. Ogilvie, “Probing photosynthetic energy and charge transfer with two-dimensional electronic spectroscopy,” J. Phys. Chem. Lett.3(4), 503–510 (2012). [CrossRef]
  15. C. H. Tseng, S. Matsika, and T. C. Weinacht, “Two-dimensional ultrafast Fourier transform spectroscopy in the deep ultraviolet,” Opt. Express17(21), 18788–18793 (2009). [CrossRef] [PubMed]
  16. C. H. Tseng, P. Sándor, M. Kotur, T. C. Weinacht, and S. Matsika, “Two-dimensional Fourier transform spectroscopy of adenine and uracil using shaped ultrafast laser pulses in the deep UV,” J. Phys. Chem. A116(11), 2654–2661 (2012). [CrossRef] [PubMed]
  17. A. Weiner, “Femtosecond pulse shaping using spatial light modulators,” Rev. Sci. Instrum.71(5), 1929–1960 (2000). [CrossRef]
  18. M. A. Montgomery, E. M. Grumstrup, and N. H. Damrauer, “Fourier transform spectroscopies derived from amplitude or phase shaping of broadband laser pulses with applications to adaptive control,” J. Opt. Soc. Am. B27(12), 2518–2533 (2010). [CrossRef]
  19. D. M. Jonas, “Two-dimensional femtosecond spectroscopy,” Annu. Rev. Phys. Chem.54(1), 425–463 (2003). [CrossRef] [PubMed]
  20. S. Mukamel, Principles of Nonlinear Optical Spectroscopy (Oxford University Press, 1995).
  21. S. M. Gallagher Faeder and D. M. Jonas, “Two-dimensional electronic correlation and relaxation spectra: theory and model calculations,” J. Phys. Chem. A103(49), 10489–10505 (1999). [CrossRef]
  22. J. Vaughan, T. Feurer, K. Stone, and K. Nelson, “Analysis of replica pulses in femtosecond pulse shaping with pixelated devices,” Opt. Express14(3), 1314–1328 (2006). [CrossRef] [PubMed]
  23. K. Blum, Density Matrix Theory and Applications, Physics of Atoms and Molecules, 2nd ed., (Plenum Press, 1996).
  24. R. W. Boyd, Nonlinear Optics, 3rd ed. (Elsevier/Academic Press, 2008).
  25. A. M. Weiner, S. DeSilvestri, and E. P. Ippen, “Three-Pulse scattering for femtosecond dephasing studies - theory and experiment,” J. Opt. Soc. Am. B2(4), 654–662 (1985). [CrossRef]
  26. H. Lee, Y.-C. Cheng, and G. R. Fleming, “Coherence dynamics in photosynthesis: Protein protection of excitonic coherence,” Science316(5830), 1462–1465 (2007). [CrossRef] [PubMed]
  27. L. Seidner, G. Stock, and W. Domcke, “Nonperturbative approach to femtosecond spectroscopy: General theory and application to multidimensional nonadiabatic photoisomerization processes,” J. Chem. Phys.103(10), 3998–4011 (1995). [CrossRef]
  28. B. Wolfseder, L. Seidner, G. Stock, and W. Domcke, “Femtosecond pump-probe spectroscopy of electron-transfer systems: a nonperturbative approach,” Chem. Phys.217(2-3), 275–287 (1997). [CrossRef]
  29. H. Wang and M. Thoss, “Nonperturbative simulation of pump–probe spectra for electron transfer reactions in the condensed phase,” Chem. Phys. Lett.389(1-3), 43–50 (2004). [CrossRef]
  30. T. S. Mančal, A. V. Pisliakov, and G. R. Fleming, “Two-dimensional optical three-pulse photon echo spectroscopy. I. Nonperturbative approach to the calculation of spectra,” J. Chem. Phys.124(23), 234504 (2006). [CrossRef] [PubMed]
  31. A. Albrecht, J. Hybl, S. Faeder, and D. Jonas, “Experimental distinction between phase shifts and time delays: Implications for femtosecond spectroscopy and coherent control of chemical reactions,” J. Chem. Phys.111(24), 10934–10956 (1999). [CrossRef]
  32. J. Hybl, Y. Christophe, and D. Jonas, “Peak shapes in femtosecond 2D correlation spectroscopy,” Chem. Phys.266(2-3), 295–309 (2001). [CrossRef]
  33. D. Jonas, (personal communication, August 10, 2011).

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