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High-harmonic and single attosecond pulse generation using plasmonic field enhancement in ordered arrays of gold nanoparticles with chirped laser pulsesYing-Ying Yang, Armin Scrinzi, Anton Husakou, Qian-Guang Li, Sarah L. Stebbings, Frederik Süßmann, Hai-Juan Yu, Seungchul Kim, Eckart Rühl, Joachim Herrmann, Xue-Chun Lin, and Matthias F. Kling »View Author Affiliations
Ying-Ying Yang,1,9
Armin Scrinzi,2
Anton Husakou,3
Qian-Guang Li,4
Sarah L. Stebbings,5
Frederik Süßmann,5
Hai-Juan Yu,1
Seungchul Kim,6
Eckart Rühl,7
Joachim Herrmann,3
Xue-Chun Lin,1
and Matthias F. Kling5,8,10
1Laboratory of solid state laser sources, Institute of Semiconductors, Chinese Academy of Sciences, Beijing, 100083, China 2Ludwig-Maximilians Universität, Theresienstrasse 37, D-80333 Munich, Germany 3Max Born Institute of Nonlinear Optics and Short Pulse Spectroscopy, Max Born Strasse 2a, D-12489 Berlin, Germany 4Department of Physics, Hubei engineering University, University, Xiaogan, 432000, China 5Max-Planck-Institut für Quantenoptik, Hans-Kopfermann-Str. 1, D-85748 Garching, Germany 6Max Planck Center for Attosecond Science (MPC-AS), POSTECH, San 31, Hyoja-Dong, Namku, Pohang, Kyungbuk 790-784, South Korea 7Institut für Chemie und Biochemie - Physikalische und Theoretische Chemie, Freie Universität Berlin, Takustr. 3, D-14195 Berlin, Germany 8J.R. Macdonald Laboratory, Physics Department, Kansas-State University, 116 Cardwell Hall, Manhattan, Kansas 66506, USA 9yangyy@semi.ac.cn 10kling@phys.ksu.edu |
Optics Express, Vol. 21, Issue 2, pp. 2195-2205 (2013)
http://dx.doi.org/10.1364/OE.21.002195
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Abstract
Coherent XUV sources, which may operate at MHz repetition rate, could find applications in high-precision spectroscopy and for spatio-time-resolved measurements of collective electron dynamics on nanostructured surfaces. We theoretically investigate utilizing the enhanced plasmonic fields in an ordered array of gold nanoparticles for the generation of high-harmonic, extreme-ultraviolet (XUV) radiation. By optimization of the chirp of ultrashort laser pulses incident on the array, our simulations indicate a potential route towards the temporal shaping of the plasmonic near-field and, in turn, the generation of single attosecond pulses. The inherent effects of inhomogeneity of the local fields on the high-harmonic generation are analyzed and discussed. While taking the inhomogeneity into account does not affect the optimal chirp for the generation of a single attosecond pulse, the cut-off energy of the high-harmonic spectrum is enhanced by about a factor of two.
© 2013 OSA
OCIS Codes
(240.6680) Optics at surfaces : Surface plasmons
(320.7110) Ultrafast optics : Ultrafast nonlinear optics
ToC Category:
Ultrafast Optics
History
Original Manuscript: November 13, 2012
Revised Manuscript: December 23, 2012
Manuscript Accepted: December 24, 2012
Published: January 22, 2013
Citation
Ying-Ying Yang, Armin Scrinzi, Anton Husakou, Qian-Guang Li, Sarah L. Stebbings, Frederik Süßmann, Hai-Juan Yu, Seungchul Kim, Eckart Rühl, Joachim Herrmann, Xue-Chun Lin, and Matthias F. Kling, "High-harmonic and single attosecond pulse generation using plasmonic field enhancement in ordered arrays of gold nanoparticles with chirped laser pulses," Opt. Express 21, 2195-2205 (2013)
http://www.opticsinfobase.org/oe/abstract.cfm?URI=oe-21-2-2195
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