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Optics Express

Optics Express

  • Editor: Andrew M. Weiner
  • Vol. 22, Iss. 16 — Aug. 11, 2014
  • pp: 19707–19725

Phonon-assisted photoluminescence from a semiconductor quantum dot with resonant electron and phonon subsystems

Anvar S. Baimuratov, Ivan D. Rukhlenko, Mikhail Yu. Leonov, Alexey G. Shalkovskiy, Alexander V. Baranov, and Anatoly V. Fedorov  »View Author Affiliations


Optics Express, Vol. 22, Issue 16, pp. 19707-19725 (2014)
http://dx.doi.org/10.1364/OE.22.019707


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Abstract

We present a theory of phonon-assisted photoluminescence from a semiconductor quantum dot (QD) whose electron and phonon subsystems are resonantly coupled via the polar electron–phonon interaction. We show that the resonance-induced renormalization of the QD energy spectrum, leading to the formation of the polaron-like states, can be performed exactly in terms of the arbitrarily degenerate states of electron–hole pairs and the phonon modes of equal energies. Using the model of QDs with finite potential barriers for electron and holes leads to new selection rules of interband optical transitions and the three-particle interaction describing simultaneous absorption and/or emission of a photon and a phonon. We also derive a simple expression for the differential cross section of the stationary, low-temperature photoluminescence, which allows the fundamental parameters of the polaron-like excitations to be readily extracted from the frequency-resolved experimental spectra. In particular, the energies of the excitations and the coherence relaxation rates of the optical transitions resulting in their generation and recombination are shown to be directly given by the positions and widths of the photoluminescence peaks. The developed theory complements the existing experimental techniques of studying the phonon-assisted photoluminescence from individual nanocrystals.

© 2014 Optical Society of America

OCIS Codes
(300.3700) Spectroscopy : Linewidth
(300.6280) Spectroscopy : Spectroscopy, fluorescence and luminescence
(300.6470) Spectroscopy : Spectroscopy, semiconductors
(160.4236) Materials : Nanomaterials
(250.5590) Optoelectronics : Quantum-well, -wire and -dot devices

ToC Category:
Spectroscopy

History
Original Manuscript: June 30, 2014
Revised Manuscript: July 24, 2014
Manuscript Accepted: July 24, 2014
Published: August 8, 2014

Citation
Anvar S. Baimuratov, Ivan D. Rukhlenko, Mikhail Yu. Leonov, Alexey G. Shalkovskiy, Alexander V. Baranov, and Anatoly V. Fedorov, "Phonon-assisted photoluminescence from a semiconductor quantum dot with resonant electron and phonon subsystems," Opt. Express 22, 19707-19725 (2014)
http://www.opticsinfobase.org/oe/abstract.cfm?URI=oe-22-16-19707


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