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Optics Express

Optics Express

  • Editor: Andrew M. Weiner
  • Vol. 22, Iss. 4 — Feb. 24, 2014
  • pp: 4388–4403

Determination of the water vapor continuum absorption by THz-TDS and Molecular Response Theory

Yihong Yang, Mahboubeh Mandehgar, and D. Grischkowsky  »View Author Affiliations


Optics Express, Vol. 22, Issue 4, pp. 4388-4403 (2014)
http://dx.doi.org/10.1364/OE.22.004388


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Abstract

Determination of the water vapor continuum absorption from 0.35 to 1 THz is reported. The THz pulses propagate though a 137 m long humidity-controlled chamber and are measured by THz time-domain spectroscopy (THz-TDS). The average relative humidity along the entire THz path is precisely obtained by measuring the difference between transit times of the sample and reference THz pulses to an accuracy of 0.1 ps. Using the measured total absorption and the calculated resonance line absorption with the Molecular Response Theory lineshape, based on physical principles and measurements, an accurate continuum absorption is obtained within four THz absorption windows, that agrees well with the empirical theory. The absorption is significantly smaller than that obtained using the van Vleck-Weisskopf lineshape with a 750 GHz cut-off.

© 2014 Optical Society of America

OCIS Codes
(010.1320) Atmospheric and oceanic optics : Atmospheric transmittance
(300.6495) Spectroscopy : Spectroscopy, teraherz
(010.1030) Atmospheric and oceanic optics : Absorption

ToC Category:
Terahertz optics

History
Original Manuscript: November 21, 2013
Revised Manuscript: February 10, 2014
Manuscript Accepted: February 11, 2014
Published: February 19, 2014

Citation
Yihong Yang, Mahboubeh Mandehgar, and D. Grischkowsky, "Determination of the water vapor continuum absorption by THz-TDS and Molecular Response Theory," Opt. Express 22, 4388-4403 (2014)
http://www.opticsinfobase.org/oe/abstract.cfm?URI=oe-22-4-4388


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